Yi Xu's research while affiliated with Jimei University and other places

Publications (37)

Article
A highly structured fluorescent-SERS dual-probe nanocomposites were synthesized for the determination of sulfur-containing gases in water and beer samples. Initially, Au@Ag NPs were prepared by growing the Ag shell on the Au core in situ, modified with surfactant and fabricated with Zn2+. Then, MOF-5-NH2 assembled Au@Ag NPs were obtained through co...
Article
A novel g-C3N4 nanosheets (g-C3N4 NSs)-assisted upconversion fluorescent aptasensor was proposed for Staphylococcus aureus (S. aureus) detection by adopting hybridization chain reaction (HCR) as a sensitizer. Two hairpin (H1 and H2) structured DNA probes were engineered predicated on the partial complementary sequence (cDNA) of S. aureus aptamer an...
Article
Food safety is regarded as a crucial factor in both human health and economic progress. This study focuses on the fabrication of a label-free surface-enhanced Raman scattering (SERS) sensor for rapid sensing of three main mycotoxins (aflatoxin B1 (AFB1), ochratoxin A (OTA), ochratoxin B (OTB)) in rice using the optimized rough silver nanoparticles...
Article
Extensively employed pesticide in agriculture causes residue in food products that would threaten public health safety. The surface-enhanced Raman scattering (SERS) signal reliant on double sensing of carbendazim and thiabendazole in a single step is achieved without the aid of any bio-recognition element. A label-free anisotropic bimetallic hollow...
Article
Nowadays, the biosensor-based detection system is developing rapidly in different fields because of the high selectivity of different recognition elements. A typical calibration needs univariate regression to correspond the value of analyte signal response with its concentrations. Although the emergence of the noninvasive biosensor, unexpected inte...
Article
Aflatoxins (AFs) contaminate agricultural products in a wide range of ways during their harvesting, storage and transport. Therefore, the detection of AFs has certain practical significance. Herein, a dispersive micro solid phase extraction (D-µSPE) technology was constructed based on 1-hexyl-3-methylimidazolium hexafluorophosphate ([HMIM][PF6]) fa...
Article
Staphylococcus aureus (S. aureus) has been identified as a marker of food contamination, closely associated with human health. This work designs a sensitive and rapid bio-detection strategy for S. aureus based on hybridization chain reaction-assisted surface enhanced Raman scattering (HCR-assisted-SERS) signal amplification. In this approach, the i...
Article
In this study, a surface enhanced Raman scattering (SERS) sensor based on [email protected] NPs solid-phase substrate combined with chemometrics was constructed for the discrimination of three pathogenic bacteria (Staphylococcus aureus, Escherichia coli and Listeria monocytogenes). The [email protected] NPs were synthesized and self-assembled on fi...
Article
Considering growing food safety issues, hollow Au/Ag nano-flower (HAu/Ag NFs) nanosensor has been synthesized for label-free and ultrasensitive detection of chloramphenicol (CP) via integrating the surface-enhanced Raman scattering (SERS) and multivariate calibration. As the anisotropic plasmonic nanomaterials, HAu/Ag NFs had numerous nano-chink on...
Article
Full-text available
Lead ion (Pb²⁺) accumulation in food consumed by humans and animals possess health threats and effects. The development of a senor for its monitoring at its minutest accumulation in edible materials becomes an antidote to safeguarding human lives. A fabricated fluorescence-based sensor made of carboxyl modified upconversion nanoparticles (UCNPs), g...
Article
The abuse of pesticides in agricultural land during pre- and post-harvest causes an increase of residue in agricultural products and pollution in the environment, which ultimately affects human health. Hence, it is crucially important to develop an effective detection method to quantify the trace amount of residue in food and water. However, with t...
Article
Pathogenic bacteria and their metabolites are the leading risk factor in food safety and are one of the major threats to human health because of the capability of triggering diseases with high morbidity and mortality. Nano-optical sensors for bacteria sensing have been greatly explored with the emergence of nanotechnology and artificial intelligenc...
Article
In this study, SERS coupled with chemometric algorithms like PLS (partial least square), Si-PLS (synergy interval-PLS), GA-PLS (genetic algorithm-PLS) and UVE-PLS (uninformative variable elimination-PLS) were applied for the detection of 2,4-D and imidacloprid in milk. The fabricated gold and silver core-shell nanoflowers ([email protected] NFs) we...
Article
A new dual-mode optical-nano-sensor was designed to effectively isolate, discriminate and inactivate multiple foodborne pathogens through the combined effort of magnetic SERS tags and functionalized upconversion nanoparticles. The positively charged quaternary ammonium salt (QAS) functionalized upconversion nanoparticles ([email protected]) were us...
Article
Considering food safety and limitations of biorecognition elements, this study focused on the development of a novel method for predicting mercury (Hg²⁺) in fish and water samples using surface-enhanced Raman scattering (SERS) coupled wavenumber selection chemometric method. Herein, core-shell [email protected] nanoparticles ([email protected] NPs)...
Article
In this study, a novel analytical approach is proposed for the identification of pesticide residues in tea by combining surface-enhanced Raman scattering (SERS) with a deep learning method one-dimensional convolutional neural network (1D CNN). First, a handheld Raman spectrometer was used for rapid on-site collection of SERS spectra. Second, the co...
Article
Pesticide residues in food have been a grave concern to consumers. Herein, we have developed a dual-mode SERS chip using Cu2O mesoporous spheres decorated with Ag nanoparticles (MCu2O@Ag NPs) as both sensing and degradation/clearing unit for rapid detection of pymetrozine and thiram pesticides in tea samples. Three kinds of chemometric algorithms w...
Article
In this study, a sensitive biosensor was developed based on aptamer functionalized polydimethylsiloxane (PDMS) film for the detection of Staphylococcus aureus (S. aureus) using surface-enhanced Raman scattering (SERS) technology. Initially, the surface of PDMS film was chemically modified by piranha solution and 3-Aminopropyltriethoxysilane (APTES)...
Article
Surface-enhanced Raman spectroscopy (SERS) has become a growing ultrasensitive analytical technique to quantify toxic molecules in foodstuffs. Monitoring the levels of chemical contaminants not only ensures food security but also offers a guideline on the production, processing, and risk analysis of consumer’s health protection. The objective of th...
Article
Trace detection of toxic chemicals in foodstuffs is of great concern in recent years. Surface-enhanced Raman scattering (SERS) has drawn significant attention in the monitoring of food safety due to its high sensitivity. This study synthesized signal optimized flower-like silver nanoparticle-(AgNP) with EF at 25 °C of 1.39×10⁶ to extend the SERS ap...
Article
Accumulation of pesticides in human body via food consumption poses health risks, hence the quantitative detection of pesticides in foodstuffs has become vital. In this study, a rapid and sensitive SERS-based sensor for detecting 2,4-dichlorophenoxyacetic acid (2,4-D) using antibody-functionalized magnetite nanoparticles (antibody-MNPs) as enrichme...
Article
Full-text available
In order to remove the limitations of natural antibodies or enzymes, a nano-magnetic biomimetic platform based on a surface-enhanced Raman scattering (SERS) sensor has been developed for highly sensitive capture and detection of 2,4-dichlorophenoxyacetic acid (2,4-D) in food and water samples. Magnetic-based molecular imprinted polymer nanoparticle...
Article
In this study, a novel sensor fabricated with compactly arranged gold nanoparticles (AuNPs) templated from mesoporous silica film (MSF) via air-water interface has been confirmed as a promising surface-enhanced Raman scattering (SERS) substrate for detecting trace levels of 2,4-dichlorophenoxyacetic acid (2,4-D), pymetrozine and thiamethoxam. The d...
Article
A highly selective and sensitive surface-enhanced Raman scattering (SERS) sensor for nitrate and nitrite determination in foodstuffs has been developed using hollow [email protected] nanosphere as a model SERS substrate. The principle of the work was based upon the significant SERS enhancement by traces of nitrite on the surface of hollow [email pr...
Article
AgNPs-plated-ZnO nanoflower (NFs)-like structures ([email protected] NFs) with optimised signals were synthesised via wet chemical method at different temperatures (50–80 °C). The enhancement factors (EFs) computed for the resultant [email protected] ranged between 2.36–8.46×10⁷ obtained at the different temperatures using 4-aminothiophenol (4-ATP)...
Article
A novel wavelength selection method namely interval combination population analysis-minimal redundancy maximal relevance (ICPA-mRMR) was employed for the trace level detection of chlorpyrifos (CPS) coupled surface-enhanced Raman spectroscopy (SERS). Herein, a highly sensitive SERS enhancement substrate Au@Ag nanoparticles (NPs) was synthesized poss...
Article
This study focused on the fabrication of a rapid, highly sensitive and inexpensive technique for the quantification of imidacloprid residue in green tea, based on surface-enhanced Raman scattering (SERS) using highly roughned surface flower shaped silver nanostructure (as SERS substrate) coupled with the chemometrics algorithm. The basic principle...
Article
With increased concerns on milk safety issues, the development of a simple and sensitive method to detect 2,4-dichlorophenoxyacetic acid (2,4-D), a common contaminant in milk, becomes relevant in safeguarding human health threats that results from its consumption. Surface-enhanced Raman spectroscopy (SERS) shows excellent ability for various target...
Article
Full-text available
Pseudomonas spp. are the dominant spoilage bacteria which can cause chicken spoilage. Some traditional detection methods are often unsuitable for their rapid real-time detection. Thus, in this paper, a fusion strategy based on colorimetric sensors and near-infrared spectroscopy was applied to rapidly identify Pseudomonas spp. in chicken. First, fou...
Article
Full-text available
This study proposed a rapid microscopic examination method for pork freshness evaluation by using the self-assembled hyperspectral microscopic imaging (HMI) system with the help of feature extraction algorithm and pattern recognition methods. Pork samples were stored for different days ranging from 0 to 5 days and the freshness of samples was divid...
Article
Mercury ion (Hg²⁺) is a highly hazardous and widespread pollutant with bio-accumulative properties. Although the existing Hg²⁺ detection methods have high sensitivity and reliability, whereas there have few reports concerning bimodal detection for Hg²⁺ with one sensor. Toward this goal, a novel sensor based on rhodamine derivatives (RhD) grafted Au...
Article
To rapidly and efficiently detect the presence of adulterants in extra-virgin olive oil, 3D fluorescence spectra technology was employed with the help of multivariate calibration. Parallel factor analysis and characteristic parameters method were comparatively employed to compress and extract the data of 3D fluorescence spectra. Then, three differe...

Citations

... Therefore, researchers have tried to use new technology to inhibit bacteria. 4,5 As it is well-known, photocatalysis is a kind of water treatment technology with high efficiency, high mineralization rate, and low cost, which provides a good strategy for tetracycline removal and bacterial inactivation. [6][7][8] Bismuth oxychloride (BiOCl) is one of the ternary bismuthbased semiconductors with a special layered structure. ...
... To on-site quantitatively measure sulfite in food, fluorescent sensors need to have the following characteristics: (1) The fluorescent sensors preferably respond to sulfite in the near-infrared (NIR) fluorescence range (650-900 nm), as the fluorescence in this range might reduce the interference of autofluorescence in food samples [33][34][35]. (2) The fluorescent sensors should exhibit a ratiometric fluorescence response to sulfite as it could effectively eliminate the fluorescence intensity errors originating from sensor distribution, excitation light intensity, photobleaching [36][37][38], etc. (3) Fluorescent sensors are better for displaying colorimetric responses to sulfite, because both fluorescence and colorimetric dual-signal responses to sulfite will make the measurement more reliable [39][40][41][42]. Therefore, the development of a colorimetric and NIR fluorescent sensor for the on-site quantitative measurement of sulfite in food samples is in great demand. ...
... Near-infrared (NIR)-excited upconversion fluorescence strategies represented by lanthanide-doped upconversion nanoparticles (UCNPs) are receiving much attention in the fields of cell imaging and tumor therapy [56]. Recently, the upconversion strategy has also been applied to HCR-based fluorescence detection of foodborne pathogens [57], where the HCR technique amplifies the strongly stabilized fluorescence signal, in addition to the NIR excitation mode, which also has the potential to penetrate deeply into food monitoring. ...
... It has been included in this section because it is a novel multiplexing strategy. Rather than directly measuring the toxins, He et al. (2023) developed a SERS-based platform for predicting content of AFB1, OTA, and ochratoxin B (OTB) in spiked rice. The procedure used 'flower-like' silver nanoparticles made with different sized polyvinylpyrrolidone polymers with K values of 15,30,and 60 (i.e. ...
... Currently, machine learning (ML) algorithms have unparalleled advantages in dealing with large sample sizes, uncovering subtle connections and complex nonlinear relationships between multiple clinical parameters and drug concentration. 19,20 ML-based models have been widely applied in pharmacy. For example, by different ML algorithms, the drug concentration is used as the output (dependent variable) and the patient's clinical parameters and demographic information, etc. are used as the inputs (covariate) to construct concentration prediction models for various drugs (tacrolimus, 21 cyclosporine, 22 teicoplanin, 23 In this study, each VCM trough concentration was treated as a separate data point and analysed independently (i.e., some patients may have >1 VCM trough concentration, each of which is processed independently). ...
... In another research study, a micro-dSPE technique was developed to extract aflatoxins from wheat and peanut samples (Zhu et al., 2022). The dispersive technique used a fabricated ZnO nanoflower sorbent in an ionic liquid. ...
... c Schematic representation of Staphylococcus aureus detection based on the target-responsive release of 4-ATP from aptamer-gated MSNs [68]. d Schematic of the Staphylococcus aureus detection based on Au@Ag/ HCR-assisted Au-magnetic [69] molecule (4-aminothiophene (4-ATP)) in aptamer-gated aminated mesoporous silica nanoparticles (MSNs) with surface-enhanced Raman scattering (SERS) technology [68]. After the aptamer recognized Staphylococcus aureus, the signal molecule 4-ATP in the MSNs hole was released, and the released SERS signal of 4-ATP was measured. ...
... In general, there have been major recent advances in clinical SERS applications for the rapid and accurate detection of bacterial pathogens [25][26][27], whereby the studies confirm the great potential of integrating SERS techniques and machine learning algorithms for the rapid and reliable identification of various bacterial pathogens, but the authors always point out the still existing wide gap between basic research and the clinical application of SERS technology. Likewise, in the food industry [28][29][30], time is crucial for product safety and a long shelf life. It might be important to mention that there are also culture-related influences on a microbial Raman spectrum, e.g. ...
... The linear dependence between the intensity of the absorption of the AuNPs-TBAP complex read at 637 nm and the CHL concentration in the range between 3.58 × 10 −6 M and 3.37 × 10 −5 M is characterized by a very good coefficient of correlation (99.44%), as presented in Figure 13. As can be concluded from the two experiments, the first one using the solely acidified TBAP-azaporphyrin and the second one being based on the same porphyrin synergistically complexed with AuNPs, these two methods are complementary, extending the detection of chloramphenicol from 3.58 × 10 −6 M to 3.37 × 10 −5 M, a domain that represents the relevant field for detecting the CHL levels in the human body fluids [65,66] and food [67][68][69], and in the industries where one must monitor for environmental control [70]. ...