April 2024
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18 Reads
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1 Citation
Applied Surface Science
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April 2024
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18 Reads
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1 Citation
Applied Surface Science
February 2024
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11 Reads
Journal of Environmental Chemical Engineering
January 2024
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32 Reads
AAPPS Bulletin
The real atomic scale details of molecular junctions would be of much complexity and can yield a plethora of “counterintuitive” results. Here, we provide an overview of four unconventional intentional or unintentional transport phenomena in molecular junctions, in particular, unconventional tunneling length-dependent transport behavior, deviation from Kirchhoff’s superposition law, dual roles of imperfect engineering, and masked quantum interference. These abnormal phenomena are not engaged in a dead end. On the contrary, it offers plenty of research opportunities in molecular electronics.
December 2023
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11 Reads
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2 Citations
Materials Today Nano
November 2023
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14 Reads
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4 Citations
Small
Oxygen vacancy defects (OVs) are one of the main strategies for nanomaterials modification to improve the photoactivity, but current methods for fabricating OVs are usually complicated and harsh. It is important to develop simple, rapid, safe, and mild methods to fabricate OVs. By studying the effects of different weak reducing agents, the concentration of the reducing agent and the reaction time on fabrication of OVs, it is found that L‐ascorbic acid (AA) gently and rapidly induces the increase of OVs in Bi4O5Br2 at room temperature. The increased OVs not only improve the adsorption of visible light, but also enhance the photocurrent response. Based on this, the preparation of OVs in Bi4O5Br2 is employed to the development of a photoelectrochemical biosensor for the detection of DNA demethylase of methyl‐CpG binding domain protein 2 (MBD2). The biosensor shows a wide linear range of 0.1–400 ng mL⁻¹ and a detection limit as low as 0.03 ng mL⁻¹ (3σ). In addition, the effect of plasticizers on MBD2 activity is evaluated using this sensor. This work not only provides a novel method to prepare OVs in bismuth rich materials, but also explores a new novel evaluation tool for studying the ecotoxicological effects of contaminants.
November 2023
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33 Reads
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1 Citation
Materials Today Physics
September 2023
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38 Reads
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2 Citations
Research on Chemical Intermediates
Nanozyme is a promising approach in treating pollution in drinking water sources. 2D MoS2 nanosheets, with abundant active sites and Lewis acid sites, exhibit outstanding peroxidase-like activity. Verified by density functional calculation, S vacancies in 2D MoS2 nanosheets can cleavage H2O to yield H⁺ and ·OH. The spontaneous generation of acid environment and oxygen free radicals enables 2D MoS2 nanosheets to be effectively exploited in the depuration of polluted water, creating a new era for multifunctional nanozymes.
September 2023
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9 Reads
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2 Citations
June 2023
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25 Reads
Nanozyme is a promising approach in treating pollution in drinking water sources. 2D MoS 2 nanosheets, with abundant active sites and Lewis acid sites, exhibits outstanding peroxidase-like and antibacterial activities. Verified by density functional calculation, S vacancies in 2D MoS 2 nanosheets can cleavage H 2 O to yield H ⁺ and ·OH. The spontaneous generation of acid environment and oxygen free radicals enables 2D MoS 2 nanosheets to be effectively exploited in the depuration of polluted water, creating a new era for multifunctional nanozymes.
January 2023
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11 Reads
... The degradation of ciprofloxacin was significantly enhanced by the photocatalytic activity of Bi/BiOF/Bi/BiOF/ Bi 2 O 2 CO 3 , which was 7 and 3.5 times greater than that of BiOF and Bi/BiOF/Bi 2 O 2 CO 3 respectively. [270] The Y-doped bismuth oxy fluoride/reduced graphene oxide (Y-BiOF/RGO) composite was synthesized using a straightforward solvothermal technique. The synthesized composite has been studied employing techniques that include transmission electron microscopy (TEM), field emission scanning electron microscopy (FESEM), photoluminescence spectroscopy (PL), UV-Vis diffuse reflectance spectroscopy (DRS), FT-IR, and X-ray diffraction (XRD). ...
December 2023
Materials Today Nano
... Generally, the total friction between layers and surfaces of layered 2D materials is composed of internal friction and edge friction. In 2D materials with small sizes, the friction is mainly caused by the edges [49,84,95,110]. Especially for heterogeneous structures, the contribution of edge atoms to friction is one to two orders of magnitude larger than that of in-plane atoms [111]. ...
November 2023
Materials Today Physics
... Supported metal catalysts are important catalysts for catalytic hydrogenation and upgrading of oil products in reducing the content of aromatics. Metal sulfides (CoMoS, NiMoS) [3][4][5] and metals (Ni, Pt, Pd) [6][7][8][9][10] were widely studied in this kind of reaction as active components. Metal sulfide catalysts can effectively improve the resistance of catalysts to sulfur, but the reaction conditions were harsh. ...
September 2023
Research on Chemical Intermediates
... Therefore, the potential of green mussel shells as a material for HA synthesis will be examined in this research. 14 Green mussel shells contain two polymorphs of calcium carbonate (CaCO 3 ), namely calcite and aragonite. 15 Most organic compounds can be found among the crystallites (intercrystalline), but some organic molecules (intercrystalline) are also intercalated in the crystal lattice. ...
November 2022
Chemical Engineering Journal
... However, dye wastewater contains a large amount of azoles and polycyclic aromatics that are challenging to degrade [2], which leads to environment pollution and serious threat to human health [3,4]. To solve those problems, various methods, including adsorption [5][6][7], flocculation [8][9][10][11], biological oxidation [12][13][14], and photodegradation [15][16][17][18] are employed. Among these, photodegradation technology has garnered significant attention due to its merits, such as high efficiency, low cost, and ease of operation [19]. ...
November 2022
Journal of Material Science and Technology
... Additionally, the photo-corrosion phenomenon can be developed due to the low migration efficiency of photo-excited charge carriers, further limiting the photocatalytic activity of Bi 5 O 7 I [90]. Fortunately, a series of adequate optimizing modifications, like semiconductor composites, noble metal doping, and surface engineering, can be harvested to strengthen solar light utilization and improve the optical properties of Bi 5 O 7 I-based heterojunction [91]. ...
August 2022
Journal of Material Science and Technology
... eV), indicating that the Fe 1 CN-20 catalyst can readily adsorb PMS molecules. This also means that PMS molecules are more easily adsorbed and activated on Fe 1 CN-20 [89]. Meanwhile, the glucose adsorption energy (E ab = -4.629 ...
August 2022
Journal of Hazardous Materials
... In Fig. 7a, the 0.2CBO/BMO curve exhibited the smallest radius, confirming that the electron transfer efficiency of 0.2CBO/BMO was greater than that of CBO and BMO. Additionally, the current density of 0.2CBO/BMO was much greater than that of CBO and BMO, providing evidence that the combination of CBO and BMO effectively promoted the migration of photogenerated carriers (Fig. 7b) [44][45][46]. Figure 8a shows the degradation curve of TC using a series of photocatalysts under visible light conditions. Prior to photocatalytic degradation, the reaction system was placed in a dark environment and stirred for 30 min to achieve adsorption equilibrium. ...
July 2022
Applied Surface Science
... After composited into the MoS 2 -Zn coatings, it remained the same antibacterial mechanism as MoS 2 particles, described as follows: Under light irradiation, MoS 2 in the MoS 2 -Zn coatings were excited, leading to the transition of e − from the valence band (VB) to the conduction band (CB), and then leaving h + on the VB. The sufficiently reducing e − on the CB of MoS 2 trapped dissolved oxygen in the water and reacted by catalytic reaction to produce the dominant active radicals ⋅O 2 - [70]. Meanwhile, H 2 O was also catalyzed by a small amount of ⋅O 2 to produce ⋅OH [71], which was tested as the subordinate active radical in the antifouling process. ...
July 2022
Separation and Purification Technology
... Liu et al. [20] prepared an in situ Z-scheme Bi 2 MoO 6 /AgI heterojunction, where the photogenerated electrons at the heterojunction interface were effectively transferred from AgI to Bi 2 MoO 6 , which exhibited excellent photocatalytic activity for the degradation of malachite green (MG). Compared with conventional heterojunction structures, p-n heterojunctions are more favorable for carrier separation due to their unique energy band structure and carrier transport properties [21,22], such as Bi 2 MoO 6 /KNbO 3 [23], BiOBr/Bi 2 MoO 6 [24], and Bi 2 MoO 6 /CuBi 2 O 4 [25]. Particularly, CuS as a conventional p-type narrow band gap semiconductor has recently attracted attention due to its excellent photoelectrochemical properties, low toxicity, and structural stability [26,27]. ...
July 2022
Separation and Purification Technology