Fengchang Wu's research while affiliated with Chinese Research Academy of Environmental Sciences and other places

Publications (565)

Article
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Biochar (BC) application to croplands aims to sequester carbon and improve soil quality, but its impact on soil organic carbon (SOC) dynamics is not represented in most land models used for assessing land-based climate change mitigation; therefore, we are unable to quantify the effects of biochar application under different climate or land manageme...
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Nutrients such as phosphorus and nitrogen lead to extensive growth of harmful algae in lakes and reservoirs, which results in eutrophication. The driving mechanism of primary productivity change in lakes and reservoirs at a wide spatial and temporal scale remains largely unknown. We establish a water quality database using a stacking machine learni...
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Lake ecosystems confront escalating challenges to their stability and resilience, most intuitively leading to biodiversity loss, necessitating effective preservation strategies to safeguard aquatic environments. However, the complexity of ecological processes governing lake biodiversity under multi-stressor interactions remains an ongoing concern,...
Article
There is still much to learn with respect to the potential for microplastics (MPs) to interact with environmental toxins and biota. In the present study, we investigated the effect of MPs on the toxicity of copper (Cu) to rice seeds ( Oryza sativa L.). The 7‐day median effective concentration (EC50) value of MPs on rice seed germination was 864 mg/...
Article
Liquid crystal monomers (LCMs) are the raw material for liquid crystal displays, and their use is steadily increasing in electronic products. Recently, LCMs have been reported to be novel endocrine disrupting chemicals, however, the mechanisms underlying their potential for thyroid hormone disruption and visual toxicity are not well understood. In...
Article
One of the fundamental objectives in ecology is to investigate the ecological processes and associated factors governing the abundance and spatial distribution patterns of biodiversity. However, the reaction of biological communities to environmental degradation remains relatively unknown, even for ecologically crucial communities like macroinverte...
Article
Due to their endocrine-disrupting effects and the risks posed in surface waters, in particular by chronic low-dose exposure to aquatic organisms, phthalate esters (PAEs) have received significant attention. However, most assessments of risks posed by PAEs were performed at a selection level, and thus limited by empirical data on toxic effects and p...
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Environmental pollution is escalating due to rapid global development that often prioritizes human needs over planetary health. Despite global efforts to mitigate legacy pollutants, the continuous introduction of new substances remains a major threat to both human and ecosystem health. In response, global initiatives are focusing on risk assessment...
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Persulfates activation by N,O-doped carbonaceous materials is an emerging advanced oxidation process for removing organic pollutants from water. However, the specific activation mechanisms including active sites, intermediates, and pathways are unknown. We prepared a N,O-doped carbocatalyst (NOGM) as model material to unveil the activation mechanis...
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Phosphorus (P) affects the water-air CO 2 flux through primary productivity, and affects the changes of carbon cycle and ecological environment in the global world. Organic phosphorus (Po) is an important P component in water environments. Various processes control the formation and transformation of Po and outbreaks of algal blooms. Here, research...
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Fenton-like catalysts are important materials for degrading refractory organic pollutants, however, they still suffer from limited oxidizing ability. Although single atoms and nanoparticles with high-index facets are commonly used in catalysis, their high surface energy hinders controllable synthesis. Here, we construct an iron-based material conta...
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Microplastic-derived dissolved organic matter(MP-DOM) exerts great effects on organiccarbon pool and its environmental behaviorsin natural waters due to increasing amountsof uncontrolled plastic disposal. However,systematic understanding of chemical com-position and environmental impacts ofMP-DOM in aquatic systems was limited. Inthis work, the che...
Article
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The spatial-temporal distribution, source, and potential ecological risk of polycyclic aromatic hydrocarbons (PAHs) in surface seawater from Laizhou Bay were investigated. The total PAH (ΣPAH) concentrations ranged from 277 to 4393 ng/L with an average of 1178 ng/L, thereby suggesting a relatively moderate to high PAH exposure level in Laizhou Bay...
Article
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Although engineered nanomaterials (ENMs) have tremendous potential to generate technological benefits in numerous sectors, uncertainty on the risks of ENMs for human health and the environment may impede the advancement of novel materials. Traditionally, the risks of ENMs can be evaluated by experimental methods such as environmental field monitori...
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Freshwater wetlands have experienced disproportionate biodiversity loss due to environmental change. The lack of long-term biological data limits our understanding of wetland biodiversity dynamics and principal drivers. Here, we combine aquatic biomonitoring with satellite-derived imagery and spatial-explicit analysis to assess the changes in macro...
Article
A variety of atmospheric lead-based chalcogenide particles (PbX n , where X = S or O) present a significant risk to environmental and public health. Foliar uptake dominates atmospheric Pb contamination of...
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Background Many studies have investigated how nanoplastics (NPs) exposure mediates nerve and intestinal toxicity through a dysregulated brain-gut axis interaction, but there are few studies aimed at alleviating those effects. To determine whether and how vitamin D can impact that toxicity, fish were supplemented with a vitamin D-low diet and vitami...
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Due to activities like mining and smelting, lead (Pb) enters the atmosphere in various forms in coarse and fine particles. It enters plants mainly through leaves, and goes up the food chain. In this study, PbXn (nano-PbS, mic-PbO and PbCl2) was applied to eggplant (Solanum melongena L.) leaves, and 379 differential metabolites were identified and a...
Article
Micropollutants in water environments have attracted widespread attention, but how human and natural stressors influence the risks of micropollutants has not been comprehensively revealed. A megacity-scale study of the ecological risks of micropollutants in the surface water of Beijing, China is presented to illustrate the magnitudes of the influen...
Article
In an urban river, comprehending the interplay between dissolved organic matter (DOM) and atmospheric, terrestrial, and aquatic sources is crucial. This encompassed investigating temporal variations in DOM and its association with the bacterioplankton community to gain profound insights into the biogeochemical dynamics and biodegradability of DOM....
Article
Organophosphate esters (OPEs) have been used worldwide as organophosphate flame retardants (OPFRs) since brominated flame retardants (BFRs) were banned. Due to the toxicity of these OPEs, environmental concerns and ecological risks arose. However, there are still large gaps in the understanding of their toxicity to organisms and the mechanisms of t...
Preprint
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The extensive application of graphene nanosheets (GNSs) has raised concerns over risks to sensitive species in the aquatic environment. The humic acid (HA) corona is traditionally considered to reduce GNSs toxicity. Here, we evaluated the effect of sorbed HA (GNSs-HA) on the toxicity of GNSs to Gram positive Bacillus tropicus . Contrary to previous...
Article
Arsenic (As) is a potentially toxic element (PTE) that causes adverse effects on human health through contamination of soil and groundwater worldwide. Biochar has captured great interest as an amendment for improving soil fertility, immobilizing PTEs, and being a carbon stabilizer. However, unlike other cationic PTEs, pristine biochar has shown uns...
Article
Hydrogen nanobubble water (HNW) is an emerging technique in the field of environment and agriculture that is attracting more attention due to its eminent characteristic. HNW exhibits a higher solution stagnation rate with a longer existence in water than molecular hydrogen, which ensures its practical usage. In this Viewpoint, the properties and ap...
Article
Degradation of organic pollutants through O2 activation catalyzed by transitional metals is challenging without addition of external chemicals and input of energy. We prepare a novel Fe based catalyst by compositing carbon, iron phosphide (FexP), iron carbide (FexC), Fe0 and Cu NPs, which can continuously activate O2 to produce high amount of 1O2,·...
Article
The production scalability and increasing demand for nano-black phosphorus materials (nano-BPs) inevitably lead to their environmental leakage, thereby raising the risk of human exposure through inhalation, ingestion, dermal, and even intravenous pathways. Consequently, a systematic evaluation of their potential impacts on human health is necessary...
Preprint
Full-text available
Biochar application in croplands aims to sequester carbon and improve soil quality, but its impact on soil organic carbon (SOC) dynamics is not represented in most land models used for assessing land-based climate mitigation, therefore we are unable to quantify the effect of biochar applications under different climate conditions or land management...
Article
Microplastics (MPs) pollution in the Yangtze River Basin (YRB) of China has grown to be a serious issue, yet there is a lack of understanding of the environmental risks of MPs in the sediment of the entire basin. This work revealed the spatial distribution characteristics of MPs in YRB sediments, and it methodically assessed the ecological risks of...
Article
Suspended sediment (SPS) is an important environmental factor in eutrophic lakes, where they may play a significant role in the microbial nitrogen cycle and thus affect the N2O source and sink function. This study investigated the correlation and corresponding microbial mechanisms between N2O emission fluxes and SPS particle sizes. N2O emission cha...
Article
Microplastic (MP) pollution in the Yangtze River Basin, China, has become an environmental issue of great concern. However, most studies on MPs have focused on a part of the Yangtze River Basin, and still lack knowledge on the risk of MPs exposure in surface waters of the whole basin. This study overviews the differences in abundance and spatial di...
Article
There are few comparative studies of chromophoric dissolved organic matter (CDOM) in humid temperate lakes. In this study, we examined the ultraviolet absorption of water sampled from temperate lakes in Japan and China. A proportional relationship was found between the dissolved organic carbon (DOC) concentration and ultraviolet absorption coeffici...
Article
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As xenobiotics in the environment, microplastics and nanoplastics have become ever-present in the environment, especially in terrestrial environment. However, a critical issue is that these anthropogenic contaminants are toxic to some terrestrial microorganisms, and the results of that toxic interaction over time can significantly impact microbial...
Preprint
Full-text available
The spatial-temporal distribution, source, and potential ecological risk of polycyclic aromatic hydrocarbons (PAHs) in surface seawater from Laizhou Bay were investigated. The total PAHs (ΣPAHs) concentration ranged from 277 to 4393 ng/L with an average of 1178 ng/L, thereby suggested a relatively moderate to high PAHs exposure level in Laizhou Bay...
Article
A ternary micro-electrolysis system consisting of carbon-coated metallic iron with Cu nanoparticles (Fe0/C@Cu0) was synthesized for the degradation of sulfathiazole (STZ). Fe0/C@Cu0 catalysts exhibited excellent reusability and stability owing to the inner tailored Fe0 with persistent activity. The connection between Fe and Cu elements in the Fe0/C...
Article
Previous studies have demonstrated that e-SOx can regulate the sedimentary release of phosphorus (P) in brackish and marine sediments. When e-SOx is active, an iron (Fe) and manganese (Mn) oxide rich layer is formed near the sediment surface, which prevents P release. When e-SOx becomes inactive, the metal oxide layer is reduced via sulfide-mediate...
Article
The increasing usage of household drugs has contributed to the widespread distribution of antibiotic pollutants in the aquatic environment. Although previous studies have proven that sediments could act as an important transport vector of antibiotic pollutants, the crucial impact of suspended sediments (SS) on the migration and fate of antibiotics...
Article
Microplastics (MPs) and their derivatives have received worldwide attention owing to their adverse effects on ecosystems. However, molecular diversity and dynamic formation of dissolved organic matter (DOM) during the photoaging of MPs remain unclear. Herein, we explored a molecular‒level formation mechanism for polystyrene MP (MPPS)‒derived DOM (P...
Article
The soil organic carbon stock (SOCS) is considered as one of the largest carbon reservoirs in terrestrial ecosystems, and small changes in soil can cause significant changes in atmospheric CO2 concentration. Understanding organic carbon accumulation in soils is crucial if China is to meet its dual carbon target. In this study, the soil organic carb...
Article
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Sustainable management of ever-increasing organic biowaste and arable soil contamination by potentially toxic elements are of concern from both environmental and agricultural perspectives. To tackle the waste issue of crawfish shells and simultaneously minimize the threat of arsenic (As) and lead (Pb) to human health, a pot trial was conducted usin...
Article
Biochar-derived dissolved black carbon (DBC) molecules are dependent on the BC formation temperature and affect the fate of emerging contaminants in waters, such as polyvinyl chloride microplastic (MPPVC). However, the temperature-dependent evolution and MPPVC-interaction of DBC molecules remain unclear. Herein, we propose a novel DBC-MPPVC interac...
Article
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Legacy per- and polyfluoroalkyl substances (PFASs) have elicited much concern because of their ubiquitous distribution in the environment and the potential hazards they pose to wildlife and human health. Although an increasing number of effective PFAS alternatives are available in the market, these alternatives bring new challenges. This paper comp...
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A comprehensive and accurate estimation of water quality in lakes and reservoirs is vital for the protection of the aquatic biota. Research on the spatiotemporal variations of nitrogen (N) and phosphorus (P) concentrations in lacustrine systems is typically plagued, however, by a lack of long‐term, spatially continuous monitoring data. This paper a...
Article
Nickel (Ni) is used primarily in the production of alloys like stainless steel and is increasingly being used in the production of batteries for the electric vehicle market. Exposure of Ni to ecosystems is of concern because Ni can be toxic to aquatic organisms. The influence of water chemistry constituents (e.g., hardness, pH, dissolved organic ca...
Article
Municipal solid waste (MSW) without proper managements could be a significant source of greenhouse gas (GHG) emissions. MSW incineration with electricity recovery (MSW-IER) is recognized as a sustainable way to utilize waste, but its effectiveness on reducing GHG emissions at the city scale in China remain unclear due to limited data of MSW composi...
Article
Increasing attention on the estimation of bioavailability of organophosphate esters (OPEs) in soil or sediment has urged the development of techniques to measure soil-/sediment-associated porewater concentrations of OPEs. In this study, we investigated the sorption dynamics of 8 OPEs to polyoxymethylene (POM) spanning one order of magnitude of aque...
Article
A predictive understanding of the source-specific (e.g., point and diffuse sources) land-to-river heavy metal (HM) loads and HM dynamics in rivers is essential for mitigating river pollution and developing effective river basin management strategies. Developing such strategies requires adequate monitoring and comprehensive models based on a solid s...
Article
In traditional soil heavy metal (HM) pollution assessment, spatial interpolation analysis is often carried out on the limited sampling points in the study area to get the overall status of heavy metal pollution. Unfortunately, in many machine learning spatial information enhancement algorithms, the additional spatial information introduced fails to...
Article
In 2011, China invested US$9.8 billion to combat the severe heavy metal pollution in the Xiang River basin (XRB), aiming to reduce 50% of the 2008 industrial metal emissions by 2015. However, river pollution mitigation requires a holistic accounting of both point and diffuse sources, yet the detailed land-to-river metal fluxes in the XRB remain unc...
Article
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Microplastics (MPs) and nanoplastics (NPs) are widely detected in food and the human environment. More studies have begun to pay attention to the influence of MPs and NPs on genetics; in particular, exposure of paternal generation to MPs and NPs on epigenetic inheritance and the offspring of animal models have attracted considerable interest. In th...
Article
With the extensive production and application of black phosphorus (BP) nanosheets, release to the environment is inevitable, which raises concerns about the fate and effects of this two-dimensional (2D) material on sensitive receptors such as environmental microbes. Although the bacterial toxicity of BP nanosheets has been demonstrated, whether the...
Article
The ability to accurately assess the health risks of contaminants is limited by the shortcomings of toxicological standards. Using organophosphate esters (OPEs) as an example, this study attempted to integrate physiologically based pharmacokinetic (PBPK)-based forward dosimetry and in vitro bioassays to assess the likelihood of contaminants inducin...
Article
Full-text available
Dissolved organic matter (DOM) contains complex molecular compounds that dominate its heterogeneous dynamics and behaviors in aquatic environments. Fourier transform ion cyclotron resonance mass spectrometry (FTICR-MS) with ultra-high resolution has proven to be effective in characterizing aquatic DOM. However, a systematic summary of molecular-lev...
Article
Environmental health and toxicology research on polystyrene nanoplastic has attracted considerable attention. However, from the perspective of ecotoxicity, the definition of polystyrene nanoplastic size has been insufficient. In this paper,...

Citations

... The continuous introduction of antibiotics into the environment by livestock farming, agriculture, and wastewater discharge raises severe environmental and public health concern [1][2][3]. Antibiotics, as typical emerging contaminants, are often incompletely degraded, which can be harmful to living organisms [4]. The long-term accumulation of antibiotic residues accelerates the propagation and transfer of antibiotic-resistant genes and antibiotic-resistant bacteria [5,6]. ...
... A series of advanced technologies, such as ultraviolet-visible spectroscopy (UV-Vis), Fourier infrared spectroscopy (FTIR), and fluorescence excitation-emission matrix (EEM) spectroscopy [21][22][23], were developed to characterize the complexation properties of DOM. In recent decades, parallel factor analysis (PARAFAC) has become a popular tool used to identify different independent groups of fluorescent components from overlapping fluorophores among the various compounds in EEM spectra [24][25][26]. This technique, combined with fluorescence quenching titration (the decrease in fluorescence due to an addition of metal), can provide more detailed information on complex binding characteristics [12,27]. ...
... Ecological risk assessment has received increasing attention in recent years, the most important of which is the determination of ecotoxicity thresholds, i.e., the maximum concentration at which ecosystems are protected is regarded as an important endpoint for evaluating ecological risk . The JPCs method were utilized to assess the ecological risk of PAEs to aquatic organisms in Chinese major water bodies (Hong et al., 2024). JPCs for each PAEs were derived to show the probability of exceedance effects of different magnitudes, combining the dispersion of PAEs levels in surface waters in China (Fig. 2) and the chronic toxic effects of PAEs on various aquatic lives (Table S1). ...
... Fungi are a large group, and their filamentous structure promotes the secretion of extracellular enzymes that can enable them to be better adapted to different environments for polymer degradation, such as dissolved organics [43,44]. Fungi seem to degrade polyethylene at a higher rate compared to bacteria [45]. ...
... By contrast, allochthonous DOM is the major component of DOM in aquatic ecosystems and is usually comprised of recalcitrant compounds transported from terrestrial ecosystems by surface runoff, streams and shallow groundwater (Gao et al., 2015). In natural aquatic environment, the abundance of allochthonous organic matter, including even the progressively more prevalent dissolved black carbon and microplastic-DOM (Li et al., 2024;Song et al., 2023;Sun et al., 2023;Yamashita et al., 2021), usually increase the molecular diversity in DOM (Hong et al., 2023), which in turn may influence DOM microbial and photo-transformation (Hu et al., 2023;Milstead et al., 2023). Phototransformation, in particular, can further feedback to alter the molecular composition of DOM and thus its microbial availability (Cory et al., 2014), thereby influencing if DOM is ultimately a carbon source or sink (Dempsey et al., 2020). ...
... Larger variation and lower recovery in the measured concentrations of ANT may be attributed to the volatility and biological activities (Mackay et al. 1997 . Generally, the solubility in the water and dissolved fraction of PAHs are considered for their toxicity evaluation presuming that only the dissolved part is bioavailable (Shi et al. 2024). In contrast, the suspended fraction is also bioavailable through adsorption and ingestion. ...
... Thorough safety evaluations are imperative before transitioning CBNs to clinical use, as certain carbon quantum dots (CQDs) and graphene derivatives have exhibited toxicity at high concentrations or with specific functionalizations, potentially leading to organ accumulation [184]. Moreover, the variability in synthesis and functionalization of carbon nanomaterials can significantly influence their biocompatibility, underscoring the need for rigorous testing on different cell types and in vivo models to establish a comprehensive safety profile [185]. ...
... Previous studies have indicated that both natural environmental factors and human activities exert varying degrees of influence on wetlands [54,55], suggesting that both likely drive changes in SMWs, which are also integral parts of wetland ecosystem. Combined with their ecological functions and characteristics, we speculated that these factors may also affect SMWs in the Yellow River Basin. ...
... Through the KG of the ER, it was found that when the ER is assessed for ecological categories, such as wetlands [47], rivers [13], and lakes [48], the assessment framework is mainly constructed from the risk source-risk receptor perspective, focusing on the impact of the natural ecological environment on the ER [16]; when the ER is assessed for ecological categories, such as croplands [6] and cities [49], the assessment framework is mainly constructed using the dimensions of disturbance and exposure of the ER, taking into account the impact of natural ecology and human activities [17]. Although the above assessment frameworks can effectively characterize the ER, they often confuse the classification or attribution of the indicators. ...
... Some studies have shown that MPs can change the migration and transformation of As by affecting soil physicochemical indexes such as pH, Fe/Mn content, organic matter content and enzyme activity [47,48,28]. According to the significant changes in the results of physicochemical indexes and enzyme activities of paddy soils containing conventional and biodegradable MPs, it can be seen that pH, Fe content, dissolved organic matter and FDA may be the reasons for the different migration and transformation effects of MPs to As. ...