Article

The influence of neighborhood-level urban morphology on PM2.5 variation based on random forest regression

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Abstract

To improve the atmospheric environment by optimizing urban morphology, this study develops a random forest (RF) model to investigate the influence of urban morphology on PM2.5 variations via the relative importance of urban morphology and the nonlinear response relationship between urban morphology and PM2.5. Two indices—reduction range (C↓) and rate (C˅) of PM2.5 concentrations—are defined to evaluate the temporal variations of PM2.5. Results show that RF models are more accurate and perform better than multiple linear regression models, with R² ranging from 0.861 to 0.936. Five out of nine urban morphological indicators have the most significant contribution to PM2.5 reduction. For each indicator, the nonlinear response relationship shows similar trends in general, despite of the difference at the higher pollution level. Building evenness index and water body area ratio have a similar response such that C↓ and C˅ sharply increase and tend to be stable when they reach at 0.05 and 8 %, respectively. With the increase in vegetated area ratio, the change of C↓ presents an inverted V-shape trend with the turning point of about 20 %; however, the change of C˅ greatly differs from the pollution level. A higher density of the low-rising buildings with one to three floors will lead to a small reduction rate but a greater reduction range of PM2.5. Floor area ratio values generally show a negative and nonlinear influence on C↓ and C˅. This study provides useful implications for planners and managers for PM2.5 reduction through neighborhood morphology optimization.

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... Our previous studies examined the influences of neighborhood green space and urban morphology on PM2.5 separately, providing evidence for the effects of urban green space coverage and morphological patterns and gray space forms on PM2.5 [18,32,35]. As a series of studies, hourly PM2.5 concentrations from 2016 to 2017 were collected from monitoring stations to ensure the consistency of PM2.5 data. ...
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This study explores the relationship between urban form at the metropolitan and neighborhood scale and fine particulate matter (PM2.5) concentrations by establishing multi-level regression models. This study has different assumptions about urban form depending on the scale used. While at the metropolitan scale, the urban form is related to the change in travel behavior, at the neighborhood scale, it is related to proximate emission sources such as roads, emissions facilities, employment centers, etc. The study shows that at the metropolitan scale, higher urban fragments, population density, and road density are associated with higher PM2.5 concentrations; higher job-resident balance and accessibility to schools are associated with lower PM2.5. At the neighborhood scale, a higher density of the nearby emission sources and higher accessibility to destinations are associated with higher PM2.5 concentrations. Urban fragments and land use mix have consistent impacts on air quality compared to preexisting studies. While population density and road density have two conflicting assumptions regarding PM2.5, in this study, the net effect of population density and road density on air quality is negative. Accessibility to destinations has different associations with PM2.5 depending on the scale of urban form measurement. At the metropolitan scale, high accessibility to destinations lessens PM2.5 concentrations by reducing vehicle distance. On the other hand, at the neighborhood scale, high accessibility to destinations makes it close to areas, which concentrate air emissions. We suggest that urban planners and decision-makers establish different strategies depending on urban form types when there are urban development plans.
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The integration of satellite-derived aerosol optical depth (AOD) and station-measured PM2.5 (particulate matter with an aerodynamic diameter of less than 2.5 μm) provides a promising approach for the monitoring of PM2.5. Previous models have generally only considered either the spatiotemporal heterogeneities of the AOD-PM2.5 relationship or the nonlinear relationship between AOD and PM2.5. In this paper, to simultaneously allow for the nonlinearity and spatiotemporal heterogeneities of the AOD-PM2.5 relationship, the geographically and temporally weighted neural network (GTWNN) model is proposed for the satellite-based estimation of ground-level PM2.5. The GTWNN model represents the nonlinear AOD-PM2.5 relationship via a generalized regression neural network, and is separately established for individual locations and times, to address the spatiotemporal heterogeneities of the AOD-PM2.5 relationship. Meanwhile, a spatiotemporal weighting scheme is incorporated in the GTWNN model to capture the local relations of samples for the training of the AOD-PM2.5 relationship. By the use of the Moderate Resolution Imaging Spectroradiometer (MODIS) AOD product, meteorological data, and MODIS normalized difference vegetation index (NDVI) data as input, the GTWNN model was verified using ground station PM2.5 measurements from China in 2015. The GTWNN model achieved sample-based cross-validation (CV) and site-based CV R² values of 0.80 and 0.79, respectively, and it outperformed the geographically and temporally weighted regression model (CV R²: 0.75 and 0.73) and the daily geographically weighted regression model (CV R²: 0.72 and 0.72). The proposed model implements the combination of geographical law and a neural network, and will be of great use for remote sensing retrieval of environmental variables.
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The complex mixtures of local emission sources and regional transportations of air pollutants make accurate PM2.5 prediction a very challenging yet crucial task, especially under high pollution conditions. A symbolic representation of spatio-temporal PM2.5 features is the key to effective air pollution regulatory plans that notify the public to take necessary precautions against air pollution. The self-organizing map (SOM) can cluster high-dimensional datasets to form a meaningful topological map. This study implements the SOM to effectively extract and clearly distinguish the spatio-temporal features of long-term regional PM2.5 concentrations in a visible two-dimensional topological map. The spatial distribution of the configured topological map spans the long-term datasets of 25 monitoring stations in northern Taiwan using the Kriging method, and the temporal behavior of PM2.5 concentrations at various time scales (i.e., yearly, seasonal, and hourly) are explored in detail. Finally, we establish a machine learning model to predict PM2.5 concentrations for high pollution events. The analytical results indicate that: (1) high population density and heavy traffic load correspond to high PM2.5 concentrations; (2) the change of seasons brings obvious effects on PM2.5 concentration variation; and (3) the key input variables of the prediction model identified by the Gamma Test can improve model's reliability and accuracy for multi-step-ahead PM2.5 prediction. The results demonstrated that machine learning techniques can skillfully summarize and visibly present the clusted spatio-temporal PM2.5 features as well as improve air quality prediction accuracy.
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Accurate and high temporal resolution predictions of fine particulate matter (PM2.5) and nitrogen oxides (NOx) concentrations are crucial for pollution control, air pollutant exposure and epidemiological studies. This study aimed to develop machine learning algorithms (MLAs)-based models for predicting hourly street-level PM2.5 and NOx concentrations at three roadside stations in Hong Kong. We comprehensively evaluated and compared the performance of six common MLAs including Random Forest (RF), Boosted Regression Trees (BRT), Support Vector Machine (SVM), Extreme Gradient Boosting (XGBoost), Generalized Additive Model (GAM), and Cubist and hence applied the most suitable MLAs to apportion the contributions from emission and non-emission factors to hourly street-level PM2.5 and NOx concentrations. The results show that RF outperforms other MLAs with ten-fold cross validation (CV) R² values higher than 0.81 and 0.62 for PM2.5 and NOx predictions, respectively. BRT, XGBoost and Cubist presented comparable predictive performance, with CV R² of 0.79–0.83 (for PM2.5 predictions) and 0.59–0.71 (for NOx predictions). SVM and GAM had worse predictions than other MLAs. The external validation R² values for RF and BRT models were more than 0.62 and 0.51 for PM2.5 and NOx concentration predictions, respectively. Non-emission factors contributed 84% and 65% to the predictions of street-level PM2.5 and NOx concentrations, respectively. Non-local pollution and temperature were the major non-emission factors, whereas private cars were the major emission contributor. This study highlights the capability of MLAs to produce high temporal resolution air pollution predictions, which can supplement traditional methods (e.g., land use regression) in generating accurate and high-temporal-resolution estimations of air pollution concentration.
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Previous studies on air pollution exposure have mostly focused on the urban, regional, national and global scales, but the outcomes cannot well support risk assessments in urban communities. To determine how the urban form and meteorology influence the air pollution distribution at a neighborhood scale (2 km*2 km), we performed a fine-scale investigation of a typical air pollutant (i.e., PM 2.5) by mobile measurements in two communities in the inner and outer cities of Shanghai, China. The PM 2.5 mass concentrations and potential impacting factors, such as PM 2.5 background levels, road networks, traffic volumes, meteorological parameters, building heights and land use types, were collected at a 10 m spatial resolution, and their relationships were analyzed using both a generalized additive model (GAM) and land use regression (LUR). The modeling results showed that the GAM outperformed LUR in both study areas, with a higher adjusted R 2 and a lower RMSE. The PM 2.5 was found to have drastic variations at the neighborhood scale, which was primarily driven by spatial patterns of the PM 2.5 background levels and traffic volumes. The GAM-based PM 2.5 concentration surface clearly disclosed the heterogeneous variation of the PM 2.5 mass concentrations in each community, and demonstrated the prominent influence from the nearby highway, especially in the central urban area. This study provides the first empirical evidence of the exposure heterogeneity of the air pollution on a neighborhood scale, which can assist planners and policymakers in evaluating planning strategies with a full consideration of reducing local air pollution.
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PM2.5 poses a serious threat to public health, however its spatial concentrations are not well characterized due to the sparseness of regulatory air quality monitoring (AQM) stations. This motivates novel low-cost methods to estimate ground-level PM2.5 at a fine spatial resolution so that PM2.5 exposure in epidemiological research can be better quantified. Satellite-retrieved aerosol products are widely used to estimate the spatial distribution of ground-level PM2.5. However, these aerosol products can be subject to large uncertainties due to many approximations and assumptions made in multiple stages of their retrieval algorithms. Therefore, estimating ground-level PM2.5 directly from satellites (e.g. satellite images) by skipping the intermediate step of aerosol retrieval can potentially yield lower errors because it avoids retrieval error propagating into PM2.5 estimation and is desirable compared to current ground-level PM2.5 retrieval methods. Additionally, the spatial resolutions of estimated PM2.5 are usually constrained by those of the aerosol products and are currently largely at a comparatively coarse 1 km or greater resolution. Such coarse spatial resolutions are unable to support scientific studies that thrive on highly spatially-resolved PM2.5. These limitations have motivated us to devise a computer vision algorithm for estimating ground-level PM2.5 at a high spatiotemporal resolution by directly processing the global-coverage, daily, near real-time updated, 3 m/pixel resolution, three-band micro-satellite imagery of spatial coverages significantly smaller than 1 × 1 km (e.g., 200 × 200 m) available from Planet Labs. In this study, we employ a deep convolutional neural network (CNN) to process the imagery by extracting image features that characterize the day-to-day dynamic changes in the built environment and more importantly the image colors related to aerosol loading, and a random forest (RF) regressor to estimate PM2.5 based on the extracted image features along with meteorological conditions. We conducted the experiment on 35 AQM stations in Beijing over a period of ∼3 years from 2017 to 2019. We trained our CNN-RF model on 10,400 available daily images of the AQM stations labeled with the corresponding ground-truth PM2.5 and evaluated the model performance on 2622 holdout images. Our model estimates ground-level PM2.5 accurately at a 200 m spatial resolution with a mean absolute error (MAE) as low as 10.1 μg m⁻³ (equivalent to 23.7% error) and Pearson and Spearman r scores up to 0.91 and 0.90, respectively. Our trained CNN from Beijing is then applied to Shanghai, a similar urban area. By quickly retraining only RF but not CNN on the new Shanghai imagery dataset, our model estimates Shanghai 10 AQM stations' PM2.5 accurately with a MAE and both Pearson and Spearman r scores of 7.7 μg m⁻³ (18.6% error) and 0.85, respectively. The finest 200 m spatial resolution of ground-level PM2.5 estimates from our model in this study is higher than the vast majority of existing state-of-the-art satellite-based PM2.5 retrieval methods. And our 200 m model's estimation performance is also at the high end of these state-of-the-art methods. Our results highlight the potential of augmenting existing spatial predictors of PM2.5 with high-resolution satellite imagery to enhance the spatial resolution of PM2.5 estimates for a wide range of applications, including pollutant emission hotspot determination, PM2.5 exposure assessment, and fusion of satellite remote sensing and low-cost air quality sensor network information.
Article
A thorough understanding of the spatiotemporal variations of PM2.5 concentrations is crucial for mitigating PM2.5 pollution with effective measures; however, few studies have investigated this issue based on the neighborhood scale. This study investigated the spatiotemporal variations of PM2.5 concentrations in 40 sites from five megacities by using hourly PM2.5 concentrations derived from air quality monitoring stations. Two relative indicators—the range and rate of change in PM2.5 concentration—were calculated to exclude the background levels of PM2.5 in different cities. Therefore, the differences between both the regions and between the sites within the same city were taken into consideration. Results showed that the within-city differences in PM2.5 concentration gradually increased from 2015 to 2017, and the differences were greater at a lower pollution level. Neighborhood-level PM2.5 concentration fluctuated mainly between 80% and 120% of each city's overall PM2.5 level. Combined with urban structure, the distribution of PM2.5 concentration during the four seasons presented three spatial patterns: the PM2.5 concentration was higher in the transition area, the PM2.5 concentration was higher in the core area than other areas, and the PM2.5 concentration had a relatively even distribution. Furthermore, the regional differences in the variations of PM2.5 concentrations depended on the PM2.5 concentrations differences among the cities; and the higher the PM2.5 pollution level, the greater was the observed regional difference. In addition, the range and rate of change in PM2.5 concentration had no significant differences among most sites at different pollution levels.
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PM2.5 (particles <2.5 μm in aerodynamic diameter) has become the primary pollutant in the air of most cities in China, and it is an important index reflecting the degree of air pollution. In this study, the response of the PM2.5 concentration in the air to multiple factors reflecting the meteorological, underlying surface and socioeconomic conditions in the Yangtze River Delta region from 2001 to 2010 was investigated by Spearman correlation analysis, multivariate analysis of variance (MANOVA) and lasso regression. In consideration of the characteristics of natural conditions and intensity of human activities in the Yangtze River Delta region, we designed six spatial scales to explore finely the effects of each factor on PM2.5 concentration. The results may provide decision support for the cross-regional air pollution risk identification. The main conclusions are as follows: (1) In different buffer zones, the dominant factors affecting the PM2.5 concentration are different. The buffer zones of 30, 40 and 50 km are the most effective areas for socioeconomic factors to affect the PM2.5 concentration. (2) The physical properties of underlying surfaces have significant effects on the PM2.5 concentration. Forestland can reduce PM2.5 concentrations in air to a certain extent, while land for construction has the opposite effect. (3) The influence of natural factors on the PM2.5 concentration in air is greater than that of socioeconomic factors in the Yangtze River Delta region, but the influence of socioeconomic factors on the PM2.5 concentration in buffer zones of 30, 40 and 50 km can not be ignored. The WS (the wind speed), PF (the proportion of forestland), PLC (the proportion of land for construction), P (the precipitation), NLI (the night light index), and PD (the population density) are the six main factors affecting the PM2.5 concentration in air.
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Urban forests play a vital role in terms of environmental quality related to particulate matter (PM) and studies on this area are increasing. This review discusses how urban forests influence atmospheric PM at three scales, including the single tree scale, stand scale and regional scale. Additionally, the PM analysis was divided into vertical and lateral directions at the stand scale. As individuals, trees capture particles mainly by the leaves, the extent of which is determined by the characteristics in foliar structure such as hair, trichomes, wax, stoma, shape and others. At the stand level, the effects of urban forest vegetation showed differences in the two directions (vertical and lateral) and the predicted values of deposition velocity in the vertical direction differed with various models, which resulted from the input of numerous influencing factors (e.g., meteorological factors, plant species, building design and others). At the regional scale, the removal capacity of atmospheric particles by urban forests was dependent on the pollution level, vegetation coverage area, leaf area index and underlying surface type. The PM removal capacity of different vegetation types was usually in the following order: coniferous forest > evergreen forest > deciduous forest. The analyses at different scales indicated that the roles of urban forests on PM could not be simply deemed positive or negative, because they need to be considered by combining various factors (e.g., plant species, meteorological condition and city planning and design) at different scales. Therefore, multi-scale analyses on the effects of atmospheric particles could help to better understand the roles of urban forests as a complex system and provide the foundation for future studies.
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Currently, urban air pollution becoming the major issue of urban physical environment in high density urban area. Many wind-calm zones or vortex zones can be formed where air pollution is retained or concentrated, which affects the environment and human health. To investigate this problem, the authors analyzed changes of wind velocity, direction, and air pollutant flow caused by changes in building height, volume, form, and density using a simulated three-dimensional (3D) conceptual model. The authors conducted an empirical study based on a representative high-density urban area. The results reveal that the actual 3D-simulated environment is complex. The wind environment changes continuously, and the retention or flow of the air pollutants changes drastically as well. The corner wind zones surrounding high-rise buildings may even generate new dust pollution due to the overly high wind speed. In this process, building height volume, layout, and orientation all significantly influence the flow and distribution of air pollution. Based on theoretical and empirical study, this paper discussed spatial planning strategies on the macroscopic city level, mesoscopic block level, and microscopic building level intended to promote the rapid dispersion of air pollutants by controlling the wind environment through optimizing the urban form.
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Aerosol optical depth (AOD) from polar orbit satellites and meteorological factors have been widely used to estimate concentrations of surface particulate matter with an aerodynamic diameter <2.5 μm (PM2.5). However, estimations with high temporal resolution remain lacking because of the limitations of satellite observations. Here, we used AOD data with a temporal resolution of 1 h provided by a geostationary satellite called Himawari 8 to overcome this problem. We developed a stacking model, which contained three submodels of machine learning, namely, AdaBoost, XGBoost and random forest, stacked through a multiple linear regression model. Then, we estimated the hourly concentrations of PM2.5 in Central and Eastern China. The accuracy evaluation showed that the proposed stacking model performed better than the single models when applied to the test set, with an average coefficient of determination (R2) of 0.85 and a root-mean-square error (RMSE) of 17.3 μg/m3. Model precision reached its peak at 14:00 (local time), with an R2 (RMSE) of 0.92 (12.9 μg/m3). In addition, the spatial and temporal distributions of PM2.5 in Central and Eastern China were plotted in this study. The North China Plain was determined to be the most polluted area in China, with an annual mean PM2.5 concentration of 58 μg/m3 during daytime. Moreover, the pollution level of PM2.5 was the highest in winter, with an average concentration of 73 μg/m3.
Article
Rapid urbanization in China has led to increasingly serious air pollution, mainly particulate matter (PM) and NOx, which has caused significant negative impacts on human health. In typical water network cities such as Wuhan, the purification of air pollution through the ecological effect of water bodies is an effective way to implement improvements. In this study, we conducted correlation analysis and established linear regression models to explore the relationship between water surface area and PM2.5, PM10, and NO2 concentrations by using pollutant monitoring data 2017, combined with water body information in remote sensing images. We found that the stability of concentration of particulate matters was low in areas where free water exists, which indicates that water has a role in absorption and minimization of PM. We also found that the concentrations of the three pollutants were strongly and negatively correlated with the free surface water coverage, with NO2 > PM2.5 > PM10, and the concentration of PM2.5, PM10 and NO2 was decreased by 2.45%, 2.96% and 9.65% respectively when water surface area increased by 10%. In addition, increasing water surface coverage in a specific size region can most effectively reduce pollutant concentrations.
Article
The rapid urbanization of China related to fine particulate (PM2.5) emissions has attracted global attention, and exploring how urban forms affect PM2.5 concentration has become a hot topic for sustainable development of cites. Here, we combined multisource data and econometric models to quantify the relationships between urban forms and PM2.5 concentration in 250 Chinese cities, with explicit consideration of urban area size, population size, economic structure, and geographical location. The results showed that urban expansion had significant positive impacts on PM2.5 concentration in medium-sized (50–150 km²) and very large-sized cities (>250 km²). Urban form compactness tended to be beneficial for the reduction in PM2.5 concentration in large cities (5 million < population < 10 million). The urban form-PM2.5 concentration relationships were also dominated by economic structure change. That is, urban form irregularity/compactness played an important role in PM2.5 concentration within second cities (the proportion of second industry > 50%) and other cities compared to third cities (the proportion of third industry > 50%). Moreover, a compact and connected urban form was found to be more beneficial for reducing PM2.5 emissions in the northern region than in other regions. This study illustrates that the urban form-PM2.5 concentration relationships are sensitive to the differences in urban types and suggests that flexible urban planning strategies can actually help to reduce PM2.5 concentration in Chinese cities.
Article
Atmospheric particulate matter (PM)pollution is becoming a growing global problem with the rapid process of urbanization. Urban green space (UGS)can effectively alleviate PM; however, few studies have investigated the effects of the UGS morphological pattern on PM, especially from a spatial strategy perspective. This study probed the contribution and strength of UGS on variation of PM 2.5 concentration based on morphological spatial pattern analysis (MSPA). Three relative indicators (range, duration, and rate)were used to represent PM 2.5 changes, and seven MSPA classes (core, islet, perforation, edge, loop, bridge, and branch)were performed to measure UGS morphological patterns. Stepwise regression analysis was used to build the PM 2.5 estimation models and partial correlation analysis was used to further analyze how well different MSPA classes influence PM 2.5 . Results showed that MSPA classes and meteorological factors combined can explain more of PM 2.5 increase variance at a high PM 2.5 level, and 40.7–81.4% for PM 2.5 reduction variance, and meteorological factors contributed more to PM 2.5 increase and reduction. Higher proportions of the core and bridge were conducive to restrict the growth and promote the reduction of PM 2.5 concentration, however, a higher proportion of perforation, islet, and edge showed opposite results. The effects of loop and branch were complex. In addition, higher air temperature and lower relative humidity were effective in reducing PM 2.5 . Wind speed, also a significant factor, had an unstable influence. The study results may provide important insights and effective spatial strategies for urban managers to mitigate PM 2.5 .
Article
A “call to action” has been issued for scholars in landscape and urban planning, natural science, and public health to conduct interdisciplinary research on the human health effects of spending time in or near greenspaces. This is timely in light of contemporary interest in municipal tree planting and urban greening, defined as organized or semi-organized efforts to introduce, conserve, or maintain outdoor vegetation in urban areas. In response to injunctions from scholars and urban greening trends, this article provides an interdisciplinary review on urban trees, air quality, and asthma. We assess the scientific literature by reviewing refereed review papers and empirical studies on the biophysical processes through which urban trees affect air quality, as well as associated models that extend estimates to asthma outcomes. We then review empirical evidence of observed links between urban trees and asthma, followed by a discussion on implications for urban landscape planning and design. This review finds no scientific consensus that urban trees reduce asthma by improving air quality. In some circumstances, urban trees can degrade air quality and increase asthma. Causal pathways between urban trees, air quality, and asthma are very complex, and there are substantial differences in how natural science and epidemiology approach this issue. This may lead to ambiguity in scholarship, municipal decision-making, and landscape planning. Future research on this topic, as well as on urban ecosystem services and urban greening, should embrace epistemological and etiological pluralism and be conducted through interdisciplinary teamwork.
Article
Airborne particulate matter (PM) has been a major threat to air quality and public health in major cities in China for more than a decade. Green space has been deemed to be effective in mitigating PM pollution; however, few studies have examined its effectiveness at the neighborhood scale. In this study, the authors probe the contributions from different landscape components in the green space (i.e., tree, grass), as well as the spatial scale of planning on fine PM (PM 2.5 ) concentrations in urban neighborhoods. PM 2.5 data including 37 samples from five megacities were collected from the National Environmental Monitoring Centre in China. Results showed that, neighborhood green space greatly contributed to the spatial variation in PM 2.5 . The total green space coverage, tree coverage, and grass coverage were all negatively correlated with PM 2.5 concentration (p < 0.05). The higher green space coverage the site had, the lower the daily mean, daily minimum, and daily maximum of PM 2.5 concentration were there. Tree coverage, in particular, was effective in reducing the PM 2.5 concentrations, and, more importantly, its effectiveness was more significant with the higher ambient PM 2.5 level. According to the examination on the effect of spatial scale, the capability for a neighborhood green space to attenuate PM 2.5 pollution would be vanished when its size smaller than 200 m, and would be maximized when its size within 400–500 m. These results will contribute to the evidence-based design and management of green space to mitigating urban PM pollution.
Article
Particulate matter with aerodynamic diameter less than 2.5 μm (PM2.5) is a complex mixture of chemical constituents emitted from various emission sources or through secondary reactions/processes; however, PM2.5 is regulated mostly based on its total mass concentration. Studies to identify the impacts on climate change, visibility degradation and public health of different PM2.5 constituents are hindered by limited ground measurements of PM2.5 constituents. In this study, national models were developed based on random forest algorithm, one of machine learning methods that is of high predictive capacity and able to provide interpretable results, to predict concentrations of PM2.5 sulfate, nitrate, organic carbon (OC) and elemental carbon (EC) across the conterminous United States from 2005 to 2015 at the daily level. The random forest models achieved high out-of-bag (OOB) R² values at the daily level, and the mean OOB R² values were 0.86, 0.82, 0.71 and 0.75 for sulfate, nitrate, OC and EC, respectively, over 2005–2015. The long-term temporal trends of PM2.5 sulfate, nitrate, OC and EC predictions agreed well with their corresponding ground measurements. The annual mean of predicted PM2.5 sulfate and EC levels across the conterminous United States decreased substantially from 2005 to 2015; while concentrations of predicted PM2.5 nitrate and OC decreased and fluctuated during the study period. The annual prediction maps captured the characterized spatial patterns of the PM2.5 constituents. The distributions of annual mean concentrations of sulfate and nitrate were generally regional in the extent that sulfate decreased from east to west smoothly with enhancement in California and nitrate had higher concentration in Midwest, Metro New York area, and California. OC and EC had regional high concentrations in the Southeast and Northwest as well as localized high levels around urban centers. The spatial patterns of PM2.5 constituents were consistent with the distributions of their emission sources and secondary processes and transportation. Hence, the national models developed in this study could provide supplementary evaluations of spatio-temporal distributions of PM2.5 constituents with full time-space coverages in the conterminous United States, which could be beneficial to assess the impacts of PM2.5 constituents on radiation budgets and visibility degradation, and support exposure assessment for regional to national health studies at county or city levels to understand the acute and chronic toxicity and health impacts of PM2.5 constituents, and consequently provide scientific evidence for making targeted and effective regulations of PM2.5 pollution.
Article
Land cover-landscape pattern affects the atmospheric environment directly or indirectly, and the understanding of the atmospheric environment response to land cover - landscape pattern is of great significance to the maintenance and improvement of ecological environment. In this paper, such 9 landscape metrics as PLAND, PD, LPI, ED, MPS, AWMSI, CONTAG, SHDI and SHEI were selected by remote sensing inversion of PM2.5 data and land use data in long time series. The correlation analysis and multiple stepwise regression analysis were also used to analyze the effect of land use and landscape pattern on PM2.5 in Yangtze River Delta. The results showed that: (1) PM2.5 concentration was increasing in Yangtze River Delta from 1998 to 2015; (2) PM2.5 concentration was negatively correlated with the forest land and grassland, while positively correlated with the urban construction land; (3) At the level of landscape type, the urban construction land, water body and farm land PLAND, LPI, ED, MPS, AWMSI were positively correlated, the urban construction land and water body PD were positively correlated with PM2.5, the farm land PD was negatively correlated with PM2.5, and the forest land and grassland PLAND, PD, LPI, ED, MPS and AWMSI were negatively correlated with PM2.5. (4) In the integral landscape of land use, AWMSI was negatively correlated with PM2.5 concentration. It is of great significance to control PM2.5 pollution from the perspective of land use planning and contributed to an estimation methods of PM2.5 concentrations using land use type and land use landscape metrics in the absence of missing PM2.5 monitoring data.
Article
In high-density cities, optimization of their compact urban forms is important for the enhancement of pollution dispersion, improvement of the air quality, and healthy urban living. This study aims to identify critical building morphological design factors and provide a scientific basis for urban planning optimization. Through a long-term mobile monitoring campaign, a four-month (spanning across summer and winter seasons) spatiotemporal street-level PM2.5 dataset was acquired. On top of that, the small-scale spatial variability of PM2.5 in the high-density downtown area of Hong Kong was mapped. Seventeen building morphological factors were also calculated for the monitoring area using geographical information system (GIS). Multivariate statistical analysis was then conducted to correlate the PM2.5 data and morphological data. The results indicate that the building morphology of the high-density environment of Hong Kong explains up to 37% of the spatial variability in the mobile monitored PM2.5. The building morphological factors with the highest correlation to PM2.5 concentration are building volume density, building coverage ratio, podium layer frontal area index and building height variability. The quantitative correlation between PM2.5 and morphological factors can be adopted to develop scientifically robust and straightforward optimization strategies for planners. This will allow considerations of pollution dispersion to be incorporated in planning practices at an early stage.
Article
Background: Daily mean concentration cannot fully address the hourly variations of air pollution within one day. As such, we proposed a new indicator, daily exceedance concentration hours (DECH), to explore the acute cardiovascular effects of ambient PM2.5 (particles with aerodynamic diameters less than 2.5μm). The DECH in PM2.5 was defined as daily total concentration-hours >25μg/m3. Methods: A generalized additive model with a quasi-Poisson link was applied to estimate the associations between day-to-day variation in PM2.5 DECH and day-to-day variation in cardiovascular mortality in six subtropical cities in Guangdong Province, China. Results: The analysis revealed significant associations between PM2.5 DECHs and cardiovascular mortality. A 500μg/m3∗h increase in PM2.5 DECHs at lag03 was associated with an increase of 4.55% (95% confidence interval (CI): 3.59%, 5.52%) in cardiovascular mortality, 4.45% (95% CI: 2.81%, 6.12%) in ischemic cardiovascular mortality, 5.02% (95% CI: 3.41%, 6.65%) in cerebrovascular mortality, and 3.00% (95% CI: 1.13%, 4.90%) in acute myocardial infarction mortality. We further observed a greater mortality burden using PM2.5 DECHs than daily mean PM2.5 (6478 (95% CI: 5071, 7917) VS 5136 (95% CI: 3990, 6305)). Conclusion: This study reveals that PM2.5 DECH is one important exposure indicator of ambient PM2.5 to measure its cardiovascular mortality effects in Pearl River Delta region; and that using daily mean concentration could under-estimate the mortality burden compared with this new indicator.
Article
The spatial-temporal characteristics of aerosol loading over the Yangtze River Basin, China during 2001–2015 were investigated using moderate resolution imaging spectroradiometer (MODIS), multi-angle imaging spectroradiometer (MISR), and ground-level particulate matter (PM) data. Aerosol optical depth (AOD) >0.8 occurs in the Yangtze River Delta, central China, and the Sichuan Basin, while AOD <0.3 occurs over higher-elevation areas in the western Sichuan Plateau and the source regions of the Yangtze River. The western Sichuan Plateau is characterized by fine-mode natural aerosols, while the source region of the Yangtze River is more influenced by dust aerosols. The Sichuan Basin, central China, and the Yangtze River Delta are dominated by anthropogenic aerosols. The spatial distribution of ground-level PM2.5 and its ratio to PM10 confirm the high aerosol loading and dominance of small particles over the middle and lower Yangtze Basin. Over the Yangtze River Delta, central China, and the Sichuan Basin, AOD varies seasonally from low in the cold months to high in the warm months, being suppressed by rainfall and wind during the Asian summer monsoon. Precipitation increases aerosol loading in the western Sichuan Plateau but reduces dust particles in the source region of the Yangtze River. There is no significant AOD trend over most areas of the Yangtze River Basin during 2001–2015, while strong decreasing trends are found over most of the middle and lower Yangtze Basin during 2011–2015. These decreasing trends may relate to changes in annual precipitation, wind speed, and air-pollution control policies. The NO2 and SO2 emissions decreased by 16.51 and 23.40% over major provinces and cities of the Yangtze River Basin from 2011 to 2015. An increase in rainfall over the middle and lower Yangtze Basin and a better pollutant diffusion condition in the Sichuan Basin also favour the decreasing AOD during this period.
Article
As the major engine of economic growth in China, the Pearl River Delta (PRD) region is one of the most urbanized regions in the world. Rapid development has brought great wealth to its citizens; however, at the same time, increasing emissions of ambient pollutants from vehicles and industrial combustions have caused considerable air pollution and negative health effects for the region's residents. In this study, the concentration response function method was applied together with satellite-retrieved particulate matter (PM10 and PM2.5) concentration data to estimate the health burden caused by this pollutant from 2004 to 2013. The value of statistical life was used to calculate the economic loss due to the negative health effects of particulate matter pollution. Our results show that in the whole PRD region, the estimated number of deaths from the four diseases attributable to PM2.5 was the highest in 2012, at 45,000 (19,000–61,000); the number of all-cause hospital admissions due to PM10 was the highest in 2013, reaching up to 91,000 (0–270,000) (excluding Hong Kong). Among the 10 cities, the capital city Guangzhou suffered the most from ambient particulate matter pollution and had the highest mortality and morbidity over the 10 years. The cost of mortality in this region was the highest in 2012, at 46,000 million USD, or around 6.1% of local total gross domestic product (GDP). The positive spatial relationship between the degree of urbanization and the particulate matter concentration proves that the urbanization process does worsen air quality and hence increases the health risks of local urban citizens. It is recommended that local governments further enhance their control policies to better guarantee the health and wealth benefits of local residents.