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Publications (151)
Accurate soil contamination delineation is crucial for deciding where remediation efforts are required. However, misjudgments, either in underestimating or overestimating
contamination extents could incur different risks: underestimation may result in environmental risks, while overestimation may lead to financial risks. This study
proposed an appr...
A crop rotation system combining agricultural production with phytoremediation is an economical and sustainable method of remediation of cadmium (Cd)-contaminated farmland. This study focuses on migration and transformation of Cd in rotation systems and the influencing factors. In a two-year field experiment, four rotation systems were evaluated: t...
Ammunition-related activities have caused severe energetic compound (EC) contamination and pose serious risks to ecosystems. However, little is known regarding the spatial-vertical variations of ECs or their migration in soils at ammunition demolition sites. Although the toxic effect of some ECs to microorganisms have been reported through laborato...
Intercropping cadmium (Cd) hyperaccumulators with crops have been widely applied in the remediation of contaminated farmland soils. However, most studies were done on drylands since the majority of the hyperaccumulators are susceptible to the aquatic environment, making the remediation of Cd-contaminated paddy fields particularly difficult. Our stu...
A low-cost practical technology is urgently needed to minimize cadmium (Cd) pollution in rice in many parts of the world. In the present study, we elucidated the effects and mechanisms of four alkaline compound materials via field experiments in southern China. The results indicated that these two alkaline Si-rich compound materials (AF-SC, alkalin...
There is a growing concern about human health of residents living in areas where mining and smelting occur. In order to understand the exposure to the potentially toxic elements (PTEs), we here identify and examine the cadmium (Cd), chromium (Cr), copper (Cu), manganese (Mn), nickel (Ni), lead (Pb) and zinc (Zn) in scalp hair of residents living in...
Soil pollution at steelworks mega-sites has become a severe environmental issue worldwide. However, due to the complex production processes and hydrogeology, the soil pollution distribution at steelworks is still unclear. This study scientifically cognized the distribution characteristics of polycyclic aromatic hydrocarbons (PAHs), volatile organic...
Rapeseed, as the most important oil crop in the world, not only affects national food security but also affects energy security and environmental security. It is very important to conduct a risk assessment of China’s rapeseed supply chain and put forward suggestions to construct a safe, effective, and accessible supply chain. In order to accurately...
This study evaluated the performance of humic acid (HA)/ferrous ion (Fe (II)) activating persulfate (PS) for fluorene (FLU) degradation. Results showed that HA/Fe(II)/PS system exhibited the best performance for PS activation to eliminate FLU. Compared to the non-activated case, the degradation efficiency of FLU had increased by 37%–43% in HA activ...
Considering the soil cadmium pollution problem, the Chinese government proposed to estimate the costs and practicality "to completely improve the soil quality by the middle of this century". This study analyzed the challenges in achieving this goal using biophysical data from 10 typical demonstration soil phytoextraction projects. The current annua...
The black soil area in Northeast China serves as a “ballast” to ensure China’s food security. Unreasonable development and utilization lead to serious black soil degradation in some areas and affect regional food production and economic and social development. In the context of the intensification of the contradiction between food supply and demand...
Vanadium (V) contamination of soils poses potential risks to humans and ecosystems. This study was conducted to evaluate the effects of endophyte-assisted phytoremediation and to determine the mechanisms involved in V detoxification and plant growth promotion. Results showed that the endophytic bacterium Serratia marcescens PRE01 could successfully...
Industrial legacies are gradually becoming an important asset for urban regeneration. Coking plants, as one of the important industrial legacies, emit large amounts of polycyclic aromatic hydrocarbons (PAHs) in production, and the health risks of PAHs in the atmosphere and soil around coking plants have been fully recognized, but not much attention...
Contamination with energetic compounds (ECs) is common in military sites and poses a great risk to the environment and human health. However, its effects on the soil bacterial communities remain unclear. This study assessed the variations of bacterial communities, co-occurrence patterns, and their influence factors in three types of typical militar...
The precision remediation and redevelopment of contaminated sites are crucial issues for improving the human settlement and constructing a beautiful China. Three-dimensional delineation of soil pollutants at contaminated sites is a prerequisite for precision remediation and redevelopment. However, a contaminated site is a three-dimensional complex...
Cadmium (Cd) contamination in rice grains has become a severe issue worldwide. This study aims to explore feasible technologies applicable to different risk lands and develop a practical solution for safe rice production at a regional scale. Despite inconsistent field conditions in the whole region, various foliar fertilizers could effectively decr...
This paper presents a novel chain model named soil–food–human (SFH) for clarifying the biogeochemical cascades among the triple challenges of cadmium contamination, food safety, and related public health effect. The model was developed based on the integration of spatial distribution pattern of soil environment and the biogeochemical process of cad...
The mining and production of mineral resources can directly lead to soil and water pollution, posing a serious threat to human health. In this study, the Taojia River basin, a tributary of the Xiangjiang River, was selected as the study area. Based on the concentrations of heavy metals (As, Cd, Pb, and Zn) in 653 soil/substrate samples collected fr...
Intense industrial activities and complex hydrogeological conditions at contaminated sites make accurate three-dimensional (3D) mapping challenging. The cause is the non-stationarity in the variance of soil pollutants in geographical space (G-space), making the stationary hypothesis required by the Kriging method unsatisfactory. To handle the varia...
The spatial association of potentially toxic elements (PTEs) in soil–crop–groundwater systems is poorly recognised. In this study, the contents of arsenic (As), cadmium (Cd), copper (Cu) and lead (Pb) in paddy soils, rice and groundwater in the Xiancha River catchment were determined. The intrinsic effects of PTEs in soils on their spatial distribu...
An analytical method of accelerated solvent extraction combined with gas chromatographic – microelectron capture detection (GC-μECD) was developed for the determination of energetic compounds (ECs) in soils from Chinese ammunition-contaminated sites. The results showed that the recoveries of most compounds were 82.86 ± 7.35 − 109.70 ± 10.82%, 82.53...
The precision remediation and redevelopment of contaminated sites are crucial for improving the living environment and constructing a beautiful China. Three-dimensional delineation of soil pollutants at contaminated sites is the basis and prerequisite for precise remediation and redevelopment. However, a contaminated site is a three-dimensional com...
Ecosystem service value (ESV) is influenced by land use and land cover (LULC), and is closely related to natural conditions and human activities. However, the interactions between human and natural systems and ESV remain unclear, especially concerning widely discussed meteorological and socioeconomic factors. In this study, three periods of LULC pa...
The pollution of Energetic compounds (ECs) in military ranges has become the focus of worldwide attention. However, few studies on the contamination of ECs at Chinese military ranges have been reported to date. In this study, two different types of military demolition range in China, Dunhua (DH) and Taiyuan (TY), were investigated and the ECs in th...
The effects of arsenate-reducing bacterial inoculants (C13, F2, F2-As and compound microbial inoculant) on the remediation of arsenic (As) contaminated soil by Pteris vittata L. were studied in field experiments. The results showed that the application of F2, F2-As and the compound microbial inoculant significantly promoted plant growth, increased...
Paddy rice agriculture in Southern China, especially Hunan Province, has been suffered from soil contamination. Several policies including rice fallow and decreasing cropping intensity have been implemented for food safety here. It is thus important to monitor rice planting area and cropping intensity to understand the effectiveness of those land-u...
Most previous studies have indicated inconsistent relationships between rice cadmium (Cd) and the soil properties of paddy fields at a regional scale under the adverse effects of confounding factors and spatial heterogeneity. In order to reduce these effects, this study integrates Geodetector, a stepwise regression model, and a hierarchical Bayesia...
The pot experiment was conducted to monitor the dynamics in soil solution chemistry in order to determine the main rhizosphere processes determining As and PAH bioavailability when utilizing P. vittata and PAH-degrading bacteria to remediate co-contaminated soils. The result showed that P. vittata was capable of depleting soil solution As and incre...
BACKGROUND
Phenanthrene (PHE) is a widespread, highly‐toxic, and biodegradable polycyclic aromatic hydrocarbon (PAH) that can be found with high concentrations in multiple industrial sites. For the efficient biodegradation of PHE, especially for the high concentrations, a PHE‐degrading Acidovorax strain was isolated from a soil contaminated for dec...
Plastic shed production system (PSPS) provide abundant vegetable products for human consumption. Comprehensive and accurate heavy metal (HM) risk assessment of soil and vegetable under plastic sheds is crucial for human health. Pollution assessment, bioavailability and mobility evaluation and health risk assessment of Cd, Cr, Cu, Zn Ni, Pb, and As...
Biochars were studied for their impacts on the dissipation and vegetable uptake of polycyclic aromatic hydrocarbons (PAHs) in an agricultural soil. The health risks of PAHs taken up by vegetables were assessed by growing Chinese cabbage in both unamended soil and biochar-amended soils. In the unamended soil, the total 16 PAHs (Σ16PAHs) content decr...
Interactive effects of inorganic arsenic (As) species and polycyclic aromatic hydrocarbons (PAHs) on their uptake, accumulation and translocation in the hyperaccumulator Pteris vittata L. (P. vittata) were studied hydroponically. The presence of PAHs hindered As uptake and acropetal translocation by P. vittata, decreasing As concentrations by 29.8%...
Heavy metal (HM) pollution of farmland is a serious problem worldwide and consumption of HM-contaminated food products poses significant public health risks. Phytoexclusion using low HM accumulating cultivars (LACs) is a promising and practical technology to mitigate the risk of HM contamination of agricultural products grown in polluted soils, and...
This study quantified influences of interactions between anthropogenic and natural factors on trace element accumulation and pollution risk in karst soils at regional and local scales and identified the dominant interacting factors. A total of 513 soil samples were collected from Hechi, southern China to measure concentrations of arsenic (As), cadm...
A number of remediation measures have been used in paddy fields to alleviate serious cadmium (Cd) contamination, which may pose a public health risk through the food chain. In this study, a field trial was conducted in paddy fields with slight–moderate Cd contamination to investigate the remediation effects of combined remediation measures (CRMs),...
In this study, we prepared polyaniline-intercalated iron oxychloride (FeOCl-PANI) by aqueous intercalation method to use it as a Fenton-like catalyst that was then assessed in terms of behavior of intercalation, structural evolution, Fenton-like activity, and catalytic mechanism. Gel-permeation chromatography demonstrated that the molecular weight...
There is great concern about the environmental impact and toxicity of palladium (Pd) because of its widespread use in automotive catalytic converters and other applications. Pd migrates and transforms in the environment and is absorbed by plant roots where it affects plant growth and eventually enters the food chain. Here we explored the effects of...
The occurrence characteristics of polycyclic aromatic hydrocarbons (PAHs) on the surfaces of buildings and devices in a typical coking plant were analyzed with the samples from different functional zones and materials. The health risk of PAHs was also evaluated. The results showed that PAHs concentrations ranged from 8.00×10-2-1.98×102 μg·dm-2, and...
Selenium (Se) and zinc (Zn) are essential microelements for humans with crucial biological functions. In this study, we determined Se and Zn concentrations in soils and rice grains on Hainan Island and investigated how their spatial distributions are related to soil mineral elements, topography, and vegetation coverage. Overall, the concentrations...
Background:
Lung cancer is the most common cancer in China. Previous studies have indicated that lung cancer incidence exhibits remarkable spatial heterogeneity, and lung cancer is related to outdoor air pollution. However, the non-linear spatial association between outdoor air pollution and lung cancer incidence in China remains unclear.
Methods...
A simple surface-enhanced Raman spectroscopy (SERS) sensor based on an undecorated gold-colloid substrate was developed for the rapid and effective detection of polycyclic aromatic hydrocarbons (PAH). The SERS enhancement of the bare Au nanoparticles for PAH was achieved by adjusting chemical reduction conditions and Cl- content. The strongest SERS...
A model integrating geo-information and self-organizing map (SOM) for exploring the database of soil environmental surveys was established. The dataset of 5 heavy metals (As, Cd, Cr, Hg, and Pb) was built by the regular grid sampling in Hechi, Guangxi Zhuang Autonomous Region in southern China. Auxiliary datasets were collected throughout the study...
The delineation of contamination at a co-contaminated site is vital for designing remedial strategy and estimating costs. Backpropagation (BP) neural networks and the Nemerow pollution index (NPI) with 3-D kriging were combined in this study to delineate contaminant plumes, analyze the spatial distribution of pollutants in different layers and visu...
To evaluate the pollution level, congener distribution, and human exposure of polybrominated diphenyl ethers (PBDEs) in the atmosphere of Beijing's office buildings, outdoor air samples (particles+gas) were collected from a typical scientific area and PBDEs concentrations were quantified using GC-MS. The results showed that the mass concentrations...
Phthalic acid esters (PAEs) as an on‐going pollution problem have attracted extensive attention due to their ubiquitous presence in the environmental medium. We investigated the distribution of six PAEs (benzyl butyl phthalate (BBP), dibutyl phthalate (DBP), di‐(2‐ethylhexyl) phthalate (DEHP), diethyl phthalate (DEP), dimethyl phthalate (DMP) and d...
Chemical oxidation is a promising pretreatment step coupled with bioremediation for removal of polycyclic aromatic hydrocarbons (PAHs). The effectiveness of Fenton, modified Fenton, potassium permanganate and activated persulfate oxidation treatments on the real contaminated soils collected from a coal gas plant (263.6 ± 73.3 mg kg ⁻¹ of the Σ16 PA...
This study mainly examines the effects of combined sieving and washing process by remediation equipment for heavy metal decontamination at a historically contaminated site. The laboratory results showed that the optimum parameters for the washing process were pH 2, 30 °C, and 10:1 liquid/soil ratio. The results from field remediation proved that th...
Accurate estimation of oxidant consumption during in situ chemical oxidation (ISCO) is the key to determining the treatment effectiveness in contaminated sites. We established the estimation model of soil oxidant demand (SOD) and simulation equations of potassium permanganate (KMnO4) dynamic consumption based on the reaction equation of KMnO4 with...
In this study, a nanocomposite material synthesized by loading nanoscale zerovalent iron (nZVI) onto biochar (BC, gasification plant byproduct) was successfully prepared, and the nZVI/BC5 (mass ratio 1:5) exhibited oxidative resistance, reutilization and stability via COD removal experiments. The nZVI/BC5 nanocomposites was used in persulfate (PS)...
This study explored the degradation effect and mechanism of persulfate oxidation activated by different macromolecular substances (polysaccharides, humic acid, and citric acid), combined with ferrous ions and different kinds of carbohydrate (monosaccharide, disaccharide, and polysaccharide). The results showed that the oxidation effects of total pe...
Removal of polycyclic aromatic hydrocarbons (PAHs) from different soil fractions of contaminated soil was investigated by using activated persulfate oxidation remediation in our research. The results showed that the light fraction, which accounted for only 10% of the soil, contained 30% of the PAHs at a concentration of 4352 mg/kg. The heavy fracti...
In this study, the removal efficiency PAHs by chemical oxidation combined with microbe remediation was evaluated in two contaminated soils. The number of indigenous soil microbes decreased after the addition of chemical oxidants and then increased by nutrients addition. The total removal efficiencies of PAHs by chemical oxidation and nutrient addit...
The nanoparticles' localized surface plasma resonance (LSPR) reveals an excellent light manipulation potentiality for the nano scale optical device development. Due to the coupling effect, the LSPR is very sensitive to the distance between the nanoparticles. Using the surface modification one nanoparticle could be grafted onto another one. But the...
A method for the remediation of polycyclic aromatic hydrocarbons (PAHs) contaminated soils was proposed involving a combination of surfactant-aided soil washing and chemical oxidation by activated persulfate (SP). In this study, Triton X-100 (TX-100) and SP was applied to the soil, either concurrently or sequentially. Results indicated that surfact...
Selenium (Se) is an essential trace element for humans. In order to investigate how soil Se is influenced by topography and soil properties, we selected Yongjia County, an area with mountainous topography, as a study area. This study used cultivated soil data to comprehensively analyze the effects of topography and soil properties on Se mobility an...
The higher values of soil and groundwater pollution index of site contamination presented a significant threat of negative impact on human health. Contamination of industrial lands has become a new environmental problem in China during the process of industrial and urbanization development. Key technologies, such as in situ chemical oxidation (ISCO...
A series of column experiments were conducted to study volatile contaminant (benzene) removal and process principles using soil vapor extraction (SVE) under different thermal conditions. Compared with the normal SVE method, two thermal methodssteam injection and electrical resistance heating effectively increased the benzene vapor diffusion and rem...
This study examined the effects of P. vittata and a polycyclic aromatic hydrocarbon (PAH)-degrading bacterium (Alcaligenes sp.) on arsenic (As) uptake and phenanthrene dissipation. Bacterial inoculation substantially increased As accumulation in plants by 27.8% (frond) and 27.5% (root) at 60d, respectively, compared with the non-inoculated treatmen...
The effects of two Pteris vittata L. accessions and a polycyclic aromatic hydrocarbon (PAH)-degrading bacterium (Alcaligenes sp.) on arsenic (As) uptake and phenanthrene dissipation were studied. The Alcaligenes sp. survived in the rhizosphere and improved soil As bioavailability with co-exposure. However, bacterial inoculation altered Pteris vitta...
In order to illuminate the mechanism of the interaction of polycyclic aromatic hydrocarbon (PAH) with different benzene rings and arsenic (As) in As hyperaccumulator, Pteris vittata L., the uptakes of PAHs were investigated using hydroponics simulation and localizations of PAHs in the plant were determined using two-photon laser scanning confocal m...
Although human biological indicators have been widely utilized for biomonitoring environmental pollutants in health exposure assessment, the relationship between internal and external exposure has not yet been adequately established. In this study, we collected and analyzed 61 rice, 56 pepper, and 58 soil samples, together with 107 hair, 107 blood,...
A framework integrating the analytic hierarchy process ( AHP) with a technique for order preference by similarity to the ideal solution ( TOPSIS) and grey evaluating ( GE) for selecting soil remediation technologies was developed and demonstrated． The methodology included two steps: 1) the establishment of an evaluation index system and weights cal...
Iron materials have shown great potential to remediate arsenic (As) contaminated sites. It’s very important to reveal the reaction process between iron materials and As from the perspective of pore scale, but relevant research was inadequate. In order to directly investigate the migration and As adsorption mechanism of starch-modified Fe-Ce oxide i...
Given great spatial variability of contaminant and depth of contamination soil in the relatively small contamination area, a three-dimensional modelling with drilling data is employed in contaminated site investigation. In order to accurately estimate the spatial distribution of soil pollution and the volume of contaminant remediation, this study p...
To ascertain absorption of arsenate and phenanthrene as well as their influence on carbon groups in excised roots of Pteris vittata L., the chemical structure of the carbon groups in excised roots was characterized by solid state ¹³C-Nuclear Magnetic Resonance (¹³C-NMR). The results showed that the excised roots could effectively absorb As and PHE...
Phytoremediation and soil washing are both potentially useful for remediating arsenic (As)-contaminated soils. We evaluated the effectiveness of a combined process coupling phytoremediation and in situ soil flushing for removal of As in contaminated soil through a pilot study. The results showed that growing Pteris vittata L. (P.v.) accompanied by...
Because of the paragenetic and associated phenomena of the mineral resources and the poor technology of mining, dressing and smelting, mine areas and their surroundings in China are polluted by various heavy metals such as arsenic, lead, cadmium, zinc, copper. Stabilization is an effective measure to solve this problem. In this manuscript, laborato...
In recent years, environmental pollution accidents occur frequently in China, which gives rise to serious environmental damage. Environmental damage identification and assessment is one of the most important environmental protection measures to cope with damage, while baseline is the key to determine the nature and extent of injuries or damages. As...
The interaction between arsenic (As) and phenanthrene (PHE) in Pteris vittata L. was investigated in this study. The migration and occurrence of PHE in P. vittata were determined by two-photon laser scanning confocal microscopy. Data indicated that PHE supplementation lowers the As concentration in P. vittata, decreasing As levels by 16.8-39.9% in...
Pteris vittata L. can absorb and accumulate high arsenic levels in soil. To clarify the occurrence characteristics of pyrene (PYR) and arsenate (As) as well as their interaction in P. vittata L., the hosting and distribution rules of PYR were determined via two-photon laser scanning confocal microscopy (TPLSCM). The results showed that PYR addition...
Batch adsorption tests and laboratory culture experiments were carried out to investigate the adsorption properties of Fe2O3, Nano-Fe2O3 and Fe-Mn binary oxides (FMBO) to arsenic (As) and stabilization effects in As-contaminated soils of different water contents. In the adsorption tests, the results showed that Pseudo-second-order kinetics model an...
Batch experiments were conducted with a heavy metals and arsenic co-contaminated soil from an abandoned mine to evaluate the feasibility of a remediation technology that combines sieving with soil washing. Leaching of the arsenic and heavy metals from the different particle size fractions was found to decrease in the order: <. 0.1, 2-0.1, and >. 2...
A pot experiment was carried out to study the effects of soil moisture on the growth and arsenic uptake of As-hyperaccumulator Pteris vittata L. The results showed that the remediation efficiency of As was the highest when the soil moisture was between 35%-45%. P. vittata grew best under 45% water content, and its aboveground and underground plant...
The Baiyun Obo deposit is the world's largest rare earth elements (REE) deposit. We aimed to investigate levels of REE, heavy metals (HMs) and uranium (U) based on morning urine samples in a population in Baiyun Obo and to assess the possible influence of rare earth mining processes on human exposure. In the mining area, elevated levels were found...
Panax notoginseng is a well-known phytomedicine used all over the world. In recent years, a certain As contamination of the herb appeared in its planting area due to elevated soil As concentration. We investigated the feasibility of intercropping with Pteris vittata, an As hyperaccumulator, on the reduction of As accumulation in Panax notoginseng a...
Experiments were carried out to investigate the effect of thermal enhanced soil vapor extraction (SVE) on benzene removal from sand, loam and clay and the mechanism. Compared to the routine control treatment, the benzene removal rates were improved by 13. 1% and 12. 3% and the remediation periods were reduced by 75% and 14%, from sand and loam resp...
An accurate assessment prior to the contaminated site remediation is essential and pre-conditional to carry out a site remediation project. In this study, a system to calculate the pollution volumetric of BaP in a contaminated site based on three-dimensional interpolation is set up to simulate the spatial distribution of soil benzopyrene (BaP) and...
Combination of hydroxyapatite (HAP) and potassium chloride (KCl) was used to stabilize lead and cadmium in contaminated mining soils. Pot experiments of chilli (Capsicum annuum) and rape (Brassica rapachinensis) were used to evaluate the stabilization efficiency. The results were the following: (1) the optimal combination decreased the leachable le...
The heavy metal and polycyclic aromatic hydrocarbons (PAHs) contents were evaluated in surface soil and plant samples of 18 wild species collected from 3 typical industrial sites in South Central China. The accumulative characteristics of the plant species for both heavy metal and PAHs were discussed. The simultaneous accumulation of heavy metal an...
Surfactant enhanced remediation is thought to be an effective method for the remediation of soils polluted with hydrophobic organic compounds. Desorption of polycyclic aromatic hydrocarbons (PAHs) from an abandoned manufactured gas plant (MGP) soil was evaluated using four eluting agents including Triton X-100 (TX100), sodium dodecylbenzene sulfona...
The problem of site contamination has become a focus in the environment protection field in the recent years. Decision support system (DSS) for remediation of contaminated sites is used for selecting the optimal remediation technologies and formulating economic and efficient remediation plans based on site investigation and risk assessment. This pa...
Panax notoginseng (Burk.) F.H. Chen, a rare traditional Chinese medicinal herb, is a widely used phytomedicine used all over the world. In recent years, the arsenic contamination of the herb and its relative products becomes a serious problem due to elevated soil As concentration. This study aimed to evaluate the effects of different types and dosa...
The influence of persulfate activation methods on polycyclic aromatic hydrocarbons (PAHs) degradation was investigated and included thermal, citrate chelated iron, and alkaline, and a hydrogen peroxide (H2O2)-persulfate binary mixture. Thermal activation (60°C) resulted in the highest removal of PAHs (99.1%) and persulfate consumption during therma...
The concentrations of 16 priority polycyclic aromatic hydrocarbons (PAHs) in four size fractions (<2, 2-20, 20-200, >200 μm) in soils at different depth from a heavily contaminated crude benzol production facility of a coking plant were determined using GC-MS. Vertically, elevated total PAHs concentrations were observed in the soils at 3.0-4.5 m (l...
