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Analysis of two-wave coupling in cubic crystal classes 23 and 4¯3m is presented for arbitrary orientation of the grating vector and the applied electric field. We show that the most efficient two-wave coupling is achieved when both the grating vector and the external electric field are parallel to the 〈1¯11〉 axis in the (110) crystal cut. However,...

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... two-wave coupling in electro-optic crystals has been studied extensively for its potentials in many applications. Much attention has been focused on materials of cubic symmetry such as the optically active sillenite crystals Bi 12 SiO 20 and Bi 12 TiO 20 ( 23 symmetry group) and the isotropic crystals GaAs, InP, and CdTe (4 ̄ 3 m symmetry group) because of their high carrier mobility, which permits achievement of fast response time. The symmetry properties of the photorefractive two-beam coupling in such crystals have been studied both theoretically and experimentally by several research groups. 1 – 5 These properties provide possibilities to realize effective energy exchange between two coherent beams in a two- wave coupling geometry, which has been demonstrated to be very useful in signal and image processing 6 and in in- terferometric measuring systems. 7 Moreover, two-beam coupling and a coherent amplification of weak beams un- derlie the photorefractive beam-fanning effect 8 that in turn is the base of photorefractive optical oscillators 9 and of both self-pumped and mutually pumped phase conjugators. 10,11 An optimal design of these devices should take into account an orientational dependence of light-induced scattering, which is mainly defined by symmetry properties of two-wave coupling. For example, the asymmetrical scattering-light distribution in a Bi 12 SiO 20 crystal under external electric field can be matched by mapping the two-wave-coupling gain of a variable grating orientation. 12 In the cited work, 12 the external electric field was parallel to the ͗ 001 ͘ axis while the interacting beams were propagating under small angles to the ͗ 110 ͘ axis. Since the early paper of Marrakchi et al. 13 this geometry was incorrectly considered as a most effective one for two-beam coupling in cubic crystals. Only six years later it was pointed out by Stepanov 14 (and confirmed by other authors 15,16 ) that the optimal geometry of two-wave coupling is achieved in these crystals when both the ex- ternal electric field and the grating vector are parallel to the ͗ ̄ 1 11 ͘ axis. Two-wave coupling in photorefractive crystals was theoretically investigated in a number of papers. 17 – 20 The most advanced theory was recently presented by Pedersen and Johansen, 21 which includes almost all effects of photorefractive beam coupling under a general angle of incidence: optical activity, externally induced linear birefringence, self diffraction, and depleted pump beam. However, this theory does not consider piezoelectric and photoelastic effects despite the importance of these effects for the explanation of the experimental results, which was pointed out by several research groups. 12,22,23 Un- fortunately, each of these works neglects one or more effects listed above. Moreover, to the best of our knowl- edge, no attempt has been made before to compare the two-wave-coupling gain for the beams propagating along the ͗ 110 ͘ axis with the counterdirectionally propagating beams. The only exception is the early paper of Fabre et al. , 24 where the particular case of the grating vector’s being parallel to the ͗ 001 ͘ axis was considered, but, as we show in this work, there is no asymmetry of the gain factor in this geometry if the counterpropagating beams are considered. The present paper is devoted to detailed theoretical and experimental study of the most effective geometry of two-wave coupling in the (110) cut of cubic crystals, when both the grating vector and the electric field are parallel to the ͗ ̄ 1 11 ͘ axis. Particularly, we demonstrate that the gain for beams propagating along the ͗ 110 ͘ axis significantly differs from the gain for the same beams but propagating backwards (along the ͗ 110 ͘ axis). If in one direction maximal beam coupling is observed for beams linearly polarized along the external electric field, then for counterpropagating beams the optimal polarization is the orthogonal one, and the net amplification is much weaker. We also show that the important peculiarities of light-induced scattering (angular distribution of the fan- out light) in sillenite crystals can be explained by mapping the two-wave-coupling gain with the obligatory con- sideration of the piezoelectric and photoelastic effects. Referring to Fig. 1, we consider the intersection of two coherent polarized beams, R and S , inside a cubic photorefractive crystal with the angle 2 ␪ between them. The bulk refractive index of the crystal is n 0 at the wavelength ␭ . These beams produce an interference pattern, which is recorded in the crystal as a space-charge-field grating with the vector K G , given by K G ϭ k R Ϫ k S , where k R and k S are the wave vectors of the beam R and S , respectively. This grating modulates the permittivity tensor of the crystal in the ...
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... k B is the Boltzmann constant, T is the absolute tem- perature, e is the electron charge, N A is the trap density, ␶ is the photoelectron lifetime, ␮ is the charge mobility, ⑀ is the low-frequency dielectric constant, ⑀ 0 is the free- space permittivity, and D is the diffusion coefficient. The optical fields R and S are assumed to be of transverse nature and these are characterized by transverse- electric and transverse-magnetic components, denoted by the subscripts E and M , respectively (see Fig. 1). R M , R E , S M , and S E are of a complex nature (to describe a general state of polarization) and are dependent on the coordinate z . 21 The modulation of the interference pattern created by these beams is given ...

Citations

... ]. Figure 5 shows the calculated distribution of the two-beam-coupling gain for BTO crystal assuming parameters, which are typical for this crystal [6]: µτ = 7 10 7 . 1 − ⋅ cm 2 ', ρ = 6.5 deg/mm, n 0 = 2.58, r 41 = 4.74 pm/V, N t = 10 22 m -3 , Λ = 20 µm, d = 2 mm, L = 10 mm, there d and L are the width and length of the crystal, respectively. ...
... The gray and black curves in Fig. 5 Difference of the two-wave-coupling gain naturally leads to the asymmetry of the DPCM efficiency, which we report here (Fig. 2). Another manifestation of the gain difference has been recently observed studying the fanning effect in BTO crystal under an alternating electric field [6]. It was found that the spatial distribution of the light-induced scattering (fanning) significantly differs whether the pump beam propagates in the direction of [110 ] axis or backward [6]. ...
... Another manifestation of the gain difference has been recently observed studying the fanning effect in BTO crystal under an alternating electric field [6]. It was found that the spatial distribution of the light-induced scattering (fanning) significantly differs whether the pump beam propagates in the direction of [110 ] axis or backward [6]. ...
... ]. Figure 5 shows the calculated distribution of the two-beam-coupling gain for BTO crystal assuming parameters, which are typical for this crystal [6]: µτ = 7 10 7 . 1 − ⋅ cm 2 ', ρ = 6.5 deg/mm, n 0 = 2.58, r 41 = 4.74 pm/V, N t = 10 22 m -3 , Λ = 20 µm, d = 2 mm, L = 10 mm, there d and L are the width and length of the crystal, respectively. ...
... The gray and black curves in Fig. 5 Difference of the two-wave-coupling gain naturally leads to the asymmetry of the DPCM efficiency, which we report here (Fig. 2). Another manifestation of the gain difference has been recently observed studying the fanning effect in BTO crystal under an alternating electric field [6]. It was found that the spatial distribution of the light-induced scattering (fanning) significantly differs whether the pump beam propagates in the direction of [110 ] axis or backward [6]. ...
... Another manifestation of the gain difference has been recently observed studying the fanning effect in BTO crystal under an alternating electric field [6]. It was found that the spatial distribution of the light-induced scattering (fanning) significantly differs whether the pump beam propagates in the direction of [110 ] axis or backward [6]. ...
Conference Paper
Full-text available
We show that a double phase-conjugate mirror recorded in photorefractive crystal of Bi12TiO20 under alternating electric field of the square-wave form possesses different efficiency for pump beams entering the crystal from opposite faces. The main reason of the observed asymmetry is a feature of the electrooptic effect in crystals of the cubic symmetry.
... The larger E 0 , the wider (in Λ) is the region of large Q. The presence of the ac-enhancement manifests itself clearly in experiments on light-induced scattering in the sillenites [16, 30, 31]: The strongest scattering angles correspond to K opt . The introduced quality factor has also an apparently different implication. ...
Article
Osnabrück, University, Diss., 2004 (Nicht für den Austausch).
Conference Paper
The sillenite crystals BSO, BTO and BGO have a great potential for real-time interferometric applications. It is important to optimize the photorefractive (PR) two-wave mixing (TWM) gain in these crystals with respect to the orientation of the grating vector and the light polarization. In Ref. ¹ it was shown that neglecting the optical activity the maximum photorefractive coupling for (1¯10)-cut crystals occurs for the grating orientation K →‖[111] and for the same (i.e. [111]) light polarization of the waves, independently of whether the piezoelectric effect is taken into account or not. Since then this conclusion has been supposed to be true also in the case of nonzero optical activity.
Conference Paper
Full-text available
http://www.opticsinfobase.org/abstract.cfm?URI=APMED-1999-SCE3 We present the main elements of an analytical theory of beam coupling in sillenites in the presence of a square-wave applied electric field. In a unified manner it includes optical activity, photo-elasticity, polarization and orientation properties and allows to describe the spatial amplification as applied to the optical configurations relevant to experiment. The main predictions of the theory are in good qualitative agreement with experimental results on light-induced scattering obtained with fiberlike BTO crystals.
Article
The effect of nonunidirectional energy exchange on the intensity and polarization state of the signal wave is analyzed in the case of symmetric two-wave coupling on a transmission photorefractive grating produced by a diffusion mechanism in a gyrotropic cubic crystal belonging to the point group 23.
Article
Theoretical and experimental investigations of the linear and nonlinear space–charge field effects in photorefractive materials are reviewed. In particular, the aim is to explore the dynamics of space–charge field formation under the influence of various enhancement mechanisms such as dc and ac electric fields, and the running holographic grating technique. Both the linear aspects and the nonlinear parametric processes are investigated. The analysis is based on the phenomenological band transport model in the single-carrier and one-step excitation version. Although many different physical effects are treated on the basis of these dynamical equations, it is demonstrated that the underlying perturbational approach appears as the governing principle both in the analytical derivations and in the physical interpretations. The principles of the recently formulated space–charge wave theory are outlined and applied to explain various nonlinear phenomena such as photorefractive parametric oscillation and amplification, and the effect of quadratic recombination.
Article
Full-text available
Mutually pumped phase conjugation with a recording time of few milliseconds is obtained in Bi 12 TiO 20 crystals by use of transient photorefractive beam coupling under a dc external electric field. It is demonstrated that the additional acceleration of the positive-feedback-loop formation is required for successful generation of transient phase-conjugate wave fronts. This acceleration is provided by the high-intensity transient photorefractive surface wave that appears immediately after application of the external electric field as the result of coupling of the incident beam with the reflected fanning beams. To the authors knowledge, this is the first experimental observation of a transient photorefractive surface wave. 1998 Optical Society of America S0740-3224(98)00807-8