(a) The Fourier spectrum of wavelength dependent THz traces pumped from 1250 nm to 2050 nm. (b) Peak-to-peak electric-field strength versus pump wavelength, showing that PNPA performs best on the range 1250 nm to 1800 nm.

(a) The Fourier spectrum of wavelength dependent THz traces pumped from 1250 nm to 2050 nm. (b) Peak-to-peak electric-field strength versus pump wavelength, showing that PNPA performs best on the range 1250 nm to 1800 nm.

Source publication
Preprint
Full-text available
We report the full characterization of a new organic nonlinear optical (NLO) crystal for intense THz generation: PNPA ((E)-4-((4-nitrobenzylidene)amino)-N-phenylaniline). We discuss crystal growth and structural characteristics. We present the wavelength dependence of THz generation, the thickness dependence of the THz spectrum for PNPA crystals, a...

Contexts in source publication

Context 1
... dependent measurements also highlight another useful aspect of PNPA. While most organic generation crystals perform best in a select range of wavelengths, PNPA generates strongly in a broad range of pump wavelengths, as shown in Figure 4. Figure 4a shows the THz spectra recorded using the 529 μm thick crystal and varying the pump wavelength from 1250 nm to 2150 nm in 100 nm steps, with a constant pump pulse energy of ~0.26 mJ. ...
Context 2
... dependent measurements also highlight another useful aspect of PNPA. While most organic generation crystals perform best in a select range of wavelengths, PNPA generates strongly in a broad range of pump wavelengths, as shown in Figure 4. Figure 4a shows the THz spectra recorded using the 529 μm thick crystal and varying the pump wavelength from 1250 nm to 2150 nm in 100 nm steps, with a constant pump pulse energy of ~0.26 mJ. In each associated spectrum, shorter pump wavelengths from 1250 nm to 1550 nm exhibit a peak in spectral amplitude at ~1.5 THz, followed by an absorption dip just above 2 THz, and significant amplitude up to higher frequencies limited by the pump pulse duration. ...
Context 3
... wavelengths from 1650 nm to 2050 nm also produce high spectral amplitudes below 2 THz, but these longer pump wavelengths appear to be better phase matched for higher THz frequencies (2-5 THz). Figure 4b shows peak-to-peak electric-field versus pump wavelength. We see that from 1250 nm to 1800 nm there is a fairly consistent peak-to-peak THz field strength, with an approximately 10% increase leading to a maximum output at 1565 nm. ...

Similar publications

Article
Full-text available
In recent days, nonlinear optical materials are getting attention because of their potential applications in the area of lasers, optical sensing and terahertz etc. A good quality single crystal of l-cysteine hydrochloride monohydrate was grown by slow evaporation solution technique using deionized water as a solvent with a time span of 25 days. The...
Article
Full-text available
Large crystal growth and characterization of the optical and terahertz (THz) properties of organic nonlinear optical (NLO) crystal NMBA (4‐Nitro‐4′‐methylbenzylidene aniline) is presented. The reported method of crystal growth consistently produces high‐quality single crystals. The THz generation efficiency and optical properties of NMBA to other T...